High performance sodium-ion full battery based on one-dimensional nanostructures: the case of Na(0.44)MnO(2)cathode and MoS(2)anode

Peng Bo; Gao Jingyu; Sun Zhihao; Li Jie; Zhang Genqiang

首页> 外文期刊>Journal of Physics, D. Applied Physics: A Europhysics Journal >High performance sodium-ion full battery based on one-dimensional nanostructures: the case of Na(0.44)MnO(2)cathode and MoS(2)anode

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High performance sodium-ion full battery based on one-dimensional nanostructures: the case of Na(0.44)MnO(2)cathode and MoS(2)anode

机译：高性能钠离子全电池基于一维纳米结构：Na（0.44）MnO（2）阴极和MOS（2）阳极的情况

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Transition metal oxides have been considered as one of the most promising cathode candidates for sodium ion batteries (SIBs). Tunnel type Na0.44MnO2, a typical cathode material for sodium ion battery, shows hopeful potential for future practical SIBs as large-scale electric energy storage system due to the low-cost and environment-friendly virtues. However, poor cyclability and rate performance of Na(0.44)MnO(2)ascribed to the slow kinetic and structural degradation have limited its practical application. Herein, single crystalline hinged nanorod shaped Na0.44MnO2(NMO-HNR) is designed by simple solid reaction. By testing the electrochemical performances of NMO-HNR samples which are synthesized at different annealing temperatures, the effects of grain size and crystallinity on electrochemical properties are investigated in detail. Thanks to the robust structure of hinged nanorod which is identified by structural and morphological characteristics after deep cycling, all the samples exhibit outstanding cyclability. Especially, the optimized NMO-HNR-900 material could deliver prominent capacity retention of 93.6% after cycling 1800 cycles at 2 A g(-1). More importantly, the full battery performance based on Na(0.44)MnO(2)cathode and MoS(2)anode is first reported in this work. As a consequence, NMO-HNR-900//Co9S8@MoS2HNT full-cell can deliver a decent cycling property with a capacity retention of 72.1% after 80 cycles.

机译：过渡金属氧化物被认为是钠离子电池（SIB）最有前途的候选阴极之一。隧道型Na0。44MnO2是一种典型的钠离子电池正极材料，具有成本低、环境友好等优点，有望成为未来实用的大规模电能存储系统。然而，由于Na（0.44）MnO（2）的缓慢动力学和结构降解，其循环性和速率性能较差，限制了其实际应用。在这里，单晶铰链纳米棒形状的Na0。44MnO2（NMO-HNR）是通过简单的固体反应设计的。通过测试在不同退火温度下合成的NMO-HNR样品的电化学性能，详细研究了晶粒尺寸和结晶度对电化学性能的影响。由于铰链纳米棒结构坚固，经过深循环后的结构和形态特征可以确定，所有样品都表现出优异的循环性能。特别是，优化后的NMO-HNR-900材料在2 A g（-1）下循环1800次后，可提供93.6%的显著容量保持率。更重要的是，本文首次报道了基于Na（0.44）MnO（2）阴极和MoS（2）阳极的全电池性能。因此，NMO-HNR-900//Co9S8@MoS2HNT全电池可提供良好的循环性能，80次循环后容量保持率为72.1%。

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《Journal of Physics, D. Applied Physics: A Europhysics Journal》 |2021年第1期|共7页
作者
Peng Bo; Gao Jingyu; Sun Zhihao; Li Jie; Zhang Genqiang;
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Univ Sci &

Technol China Hefei Natl Lab Phys Sci Microscale CAS Key Lab Mat Energy Convers Dept Mat Sci &

Engn Hefei 230026 Anhui Peoples R China;

Univ Sci &

Technol China Hefei Natl Lab Phys Sci Microscale CAS Key Lab Mat Energy Convers Dept Mat Sci &

Engn Hefei 230026 Anhui Peoples R China;

Univ Sci &

Technol China Dept Chem Hefei 230026 Anhui Peoples R China;

Univ Sci &

Technol China Hefei Natl Lab Phys Sci Microscale CAS Key Lab Mat Energy Convers Dept Mat Sci &

Engn Hefei 230026 Anhui Peoples R China;

Univ Sci &

Technol China Hefei Natl Lab Phys Sci Microscale CAS Key Lab Mat Energy Convers Dept Mat Sci &

Engn Hefei 230026 Anhui Peoples R China;

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原文格式 PDF
正文语种 eng
中图分类应用物理学;
关键词
sodium ion battery; tunnel Na0.44MnO2; one-dimension; cathode; anode;

机译：钠离子电池;隧道Na0.44mNO2;一维;阴极;阳极;

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1. Improved Electrochemical Performance Based on Nanostructured SnS2@CoS2–rGO Composite Anode for Sodium-Ion Batteries [J] . Xia Wang, Xueying Li, Qiang Li, 纳微快报：英文版 . 2018,第003期
2. 3D hierarchical microspheres constructed by ultrathin MoS2-C nanosheets as high-performance anode material for sodium-ion batteries [J] . Wenlong Zhang, Haihui Zhou, Zhongyuan Huang, 天然气化学（英文版） . 2020,第010期
3. 3D hierarchical microspheres constructed by ultrathin MoS2-C nanosheets as high-performance anode material for sodium-ion batteries [J] . Wenlong Zhang, Haihui Zhou, Zhongyuan Huang, 能源化学：英文版 . 2020,第010期
4. Towards high-performance anodes:Design and construction of cobalt-based sulfide materials for sodium-ion batteries [J] . Baole Guan, Si-Yu Qi, Ying Li, 能源化学：英文版 . 2021,第003期
5. High-rate performance electrospun Na0.44MnO2 nanofibers as cathode material for sodium-ion batteries [J] . Fu Bi, Zhou Xuan, Wang Yaping Journal of power sources . 2016,第Apra1期

机译：高性能电纺Na0.44MnO2纳米纤维作为钠离子电池的阴极材料
6. High-performance aqueous rechargeable sulfate- and sodium-ion battery based on polypyrrole-MWCNT core-shell nanowires and Na_(0.44)MnO_2 nanorods [J] . Lim Hana, Jung Ji Hea, Park Young Min, Applied Surface Science . 2018,第JULa15期

机译：基于聚吡咯-MWCNT核壳纳米线和Na_（0.44）MnO_2纳米棒的高性能水性可充电硫酸盐和钠离子电池
7. High-Performance Na 0.44 MnO 2 Slabs for Sodium-Ion Batteries Obtained through Urea-Based Solution Combustion Synthesis [J] . Chiara Ferrara, Cristina Tealdi, Valentina Dall’Asta, Batteries . 2018,第1期

机译：通过尿素基溶液燃烧合成获得的钠离子电池用高性能Na 0.44 MnO 2平板
8. Spherical MoS_2/Carbon Composite with Improved Electrochemical Performance for Sodium-Ion Battery Anode [C] . Hyojun Lim, Hyeongwoo Kim, Sang-Ok Kim, Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

机译：球形MOS_2 /碳复合材料，具有改进的钠离子电池阳极电化学性能
9. Beyond Conventional Cathode Materials for Lithium-ion Batteries and Sodium-ion Batteries Nickel fluoride conversion materials and P2 type Sodium-ion intercalation cathodes. [D] . Lee, Dae Hoe. 2013

机译：除了用于锂离子电池和钠离子电池的常规阴极材料以外，氟化镍转换材料和P2型钠离子嵌入阴极。
10. Improved Electrochemical Performance Based on Nanostructured SnS2@CoS2–rGO Composite Anode for Sodium-Ion Batteries [O] . Xia Wang, Xueying Li, Qiang Li, -1

机译：基于纳米结构的SnS2 @ CoS2–rGO复合阳极的钠离子电池电化学性能的改善
11. Durable high-rate capability Na$_{0.44}$ MnO$_{2}$ cathode material for sodium-ion batteries [O] . He, Xin, Wang, Jun, Meng, Y. Shirley, 2016

机译：耐用，高倍率的钠离子电池用Na $ _ {0.44} $ MnO $ _ {2} $正极材料
12. Theoretical Study of Si(x) Ge(y)Li(z) (x=4-10, y=1-10, z=0-10) Clusters for Designing of Novel Nanostructured Materials to be Utilized as Anodes for Lithium-Ion Batteries. [R] . Perez-Peralta, N., Sanchez-Vazquez, M. 2015

机译：si（x）Ge（y）Li（z）（x = 4-10，y = 1-10，z = 0-10）团簇的理论研究用于设计新型纳米结构材料用作锂离子阳极电池。

High performance sodium-ion full battery based on one-dimensional nanostructures: the case of Na(0.44)MnO(2)cathode and MoS(2)anode

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