Guided Lithium Deposition by Surface Micro‐Patterning of Lithium‐Metal Electrodes

Kim Yun‐Jung; Jin Hyun S.; Lee Dong‐Hyun; Choi Jaeho; Jo Wonhee; Noh Hyungjun; Lee Jinhong; Chu Hyunwon; Kwack Hobeom; Ye Fangmin; Lee Hongkyung; Ryou Myung‐Hyun; Kim Hee‐Tak

摘要

Abstract > Uncontrolled lithium (Li) deposition has hampered the evolution of Li‐metal electrode‐based Li‐batteries. In this work, we report the differences of a guided Li deposition with a size change of the square hole micro‐patterns carved on the Li‐metal surface with two different dimensions using a simple stamping method. Li deposition is preferentially initiated on the top edge for the smaller pattern and on the bottom for the larger pattern. Although the two patterns lead to a more uniform utilization of the Li, the larger pattern shows a higher cycling stability within a LiFePO <sub>4</sub> /Li cell than that of the smaller one indicating that initiating the Li deposition from the bottom of the hole is more efficient in confining the deposited Li. Based on the impedance analysis of the compressed Li electrodes, we suggest that the guided Li deposition on the bottom of the hole is attributed to a large contrast in the resistance of native surface passivation layer between the top and hole surfaces. This improved understanding can further advance guided Li deposition induced by surface patterns for high performance Li‐metal batteries. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span>None </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2018年第21期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Yun‐Jung&option=202" target="_blank" rel="nofollow">Kim Yun‐Jung;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jin Hyun S.&option=202" target="_blank" rel="nofollow">Jin Hyun S.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Dong‐Hyun&option=202" target="_blank" rel="nofollow">Lee Dong‐Hyun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Choi Jaeho&option=202" target="_blank" rel="nofollow">Choi Jaeho;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jo Wonhee&option=202" target="_blank" rel="nofollow">Jo Wonhee;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Noh Hyungjun&option=202" target="_blank" rel="nofollow">Noh Hyungjun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Jinhong&option=202" target="_blank" rel="nofollow">Lee Jinhong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chu Hyunwon&option=202" target="_blank" rel="nofollow">Chu Hyunwon;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kwack Hobeom&option=202" target="_blank" rel="nofollow">Kwack Hobeom;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ye Fangmin&option=202" target="_blank" rel="nofollow">Ye Fangmin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Hongkyung&option=202" target="_blank" rel="nofollow">Lee Hongkyung;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ryou Myung‐Hyun&option=202" target="_blank" rel="nofollow">Ryou Myung‐Hyun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Hee‐Tak&option=202" target="_blank" rel="nofollow">Kim Hee‐Tak;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> <p>Energy and Environment DirectoratePacific Northwest National Laboratory902 Battelle Boulevard Richland WA 99354 USA;</p> <p>Department of Chemical and Biological EngineeringHanbat National University125 Dongseo-daero Yuseong-gu Daejeon 34158 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology291 Daehak-ro Yuseong-gu Daejeon 34141 Republic of Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lithium&option=203" rel="nofollow">Lithium;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-metal batteries&option=203" rel="nofollow">lithium-metal batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=materials science&option=203" rel="nofollow">materials science;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=micro-patterns&option=203" rel="nofollow">micro-patterns;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=native passivation film&option=203" rel="nofollow">native passivation film;</a> </p> <div class="translation"> 机译：锂;锂金属电池;材料科学;微观图案;本机钝化膜; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a 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Sci. 1/2021)</a> <b>[O] </b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Woo Hyeong Sim&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Woo Hyeong Sim,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hyung Mo Jeong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Hyung Mo Jeong </a> <span>2020</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂金属电极：高性能锂金属电池有序氮螯合锂离子的高效锂生长控制（ADV。SCI。1/2021）</span> </p> </li> <li> <div> <b>11. </b><a class="enjiyixqcontent" href="/open-access_resources_thesis/01000126425967.html">Cover Feature: Guided Lithium Deposition by Surface Micro-Patterning of Lithium-Metal Electrodes (ChemElectroChem 21/2018)</a> <b>[O] </b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yun-Jung Kim&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yun-Jung Kim,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hyun S. Jin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Hyun S. Jin,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dong-Hyun Lee&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dong-Hyun Lee,</a> <span>2018</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：封面特征：通过锂 - 金属电极表面微图案化引导锂沉积（ChemelectoChem 21/2018）</span> </p> </li> <li> <div> <b>12. </b><a class="enjiyixqcontent" href="/ntis-science-report_ad_thesis/020711125123.html">Characterization of Lithium Electrode Surface in Lithium Secondary Batteries byIn situ Raman Spectroscopic Methods</a> <b>[R] </b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tachikawa, H.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Tachikawa, H. </a> <span>1993</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用原位拉曼光谱法表征锂二次电池中锂电极表面</span> </p> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_geology-anhui_thesis/0201290870167.html">Dendrite-Free and Stable Lithium Metal Battery Achieved by a Model of Stepwise Lithium Deposition and Stripping</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tiancun Liu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . Tiancun Liu</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jinlong Wang&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,Jinlong Wang</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yi Xu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,Yi Xu</a> <span> <a href="/journal-cn-15126/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 安徽地质 </a> </span> <span> . 2021</span><span>,第011期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-66193_thesis/020222969075.html">可判定的一阶片段Lithium逻辑研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=闫佳亮&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 闫佳亮</a> <span> <a href="/conference-cn-66193/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2017年全国现代逻辑学术研讨会 </a> <span> <span> . 2017</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020316281540.html">Deposition of Zn(Mn,Mo)--Ni--Co ternary transition metal sulfides and reduced graphene oxide on Ni foam as electrode materials for asymmetric supercapacitors</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=UWAMAHORO EVARLSTE&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . UWAMAHORO EVARLSTE</a> <span> . 2019</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120101288879.html">锂复合氧化物{Lithium complex oxide}</a> <b>[P]</b> . <span> 中国专利： CN110400915A </span> <span> . 2019-11-01</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06130500628035.html">SURFACE TREATMENT METHOD FOR LITHIUM METAL NEGATIVE ELECTRODE, SURFACE-TREATED LITHIUM METAL NEGATIVE ELECTRODE, AND LITHIUM METAL BATTERY COMPRISING SAME</a> <b>[P]</b> . <span> 外国专利：  EP3879604A1 </span> <span> . 2021-09-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂金属负极的表面处理方法，表面处理锂金属负极和包含相同的锂金属电池 </span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130400947478.html">SURFACE TREATMENT METHOD FOR LITHIUM METAL NEGATIVE ELECTRODE, SURFACE-TREATED LITHIUM METAL NEGATIVE ELECTRODE, AND LITHIUM METAL BATTERY COMPRISING SAME</a> <b>[P]</b> . <span> 外国专利：  WO2020096091A1 </span> <span> . 2020-05-14</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂金属负极的表面处理方法，表面处理过的锂金属负极和包含其的锂金属电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130424020440.html">LITHIUM METAL SOLID BODY, LITHIUM METAL FILM MADE OF THE SAME, SOLID ELECTROLYTE MEMBRANE-LITHIUM ELECTRODE ASSEMBLY INCLUDING THE METAL FILM, LITHIUM AIR BATTERY PROVIDED WITH THE SOLID ELECTROLYTE MEMBRANE-LITHIUM ELECTRODE ASSEMBLY, AND METHOD FOR MANUFACTURING THE SOLID ELECTROLYTE MEMBRANE-LITHIUM ELECTRODE ASSEMBLY</a> <b>[P]</b> . <span> 外国专利：  JP2012150909A </span> <span> . 2012-08-09</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：锂金属固体，由相同金属制成的锂膜，包括金属膜的固体电解质膜-锂电极组件，由固体电解质膜电解质膜-电解质膜制成的锂空气电池和方法部件 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704028366921','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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