Direct C-H Arylation Meets Perovskite Solar Cells: Tin-Free Synthesis Shortcut to High-Performance Hole-Transporting Materials

Chang Yu-Chieh; Lee Kun-Mu; Lai Chia-Hsin; Liu Ching-Yuan

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Direct C-H Arylation Meets Perovskite Solar Cells: Tin-Free Synthesis Shortcut to High-Performance Hole-Transporting Materials

机译：直接C-H芳基化符合Perovskite太阳能电池：无酸合成快捷速度，高性能孔输送材料

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In contrast to the traditional multistep synthesis, we demonstrate herein a two-step synthesis shortcut to triphenylamine-based hole-transporting materials (HTMs) through sequential direct C-H arylations. These hole-transporting molecules are fabricated in perovskite-based solar cells (PSCs) that exhibit promising efficiencies up to 17.69%, which is comparable to PSCs utilizing commercially available 2,2,7,7-tetrakis[N,N-di(4-methoxyphenyl)amino]-9,9-spirobifluorene (spiro-OMeTAD) as the HTM. This is the first report describing the use of step-saving C-H activations/arylations in the facile synthesis of small-molecule HTMs for perovskite solar cells.

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来源
《Chemistry, an Asian journal》 |2018年第11期|共6页
作者
Chang Yu-Chieh; Lee Kun-Mu; Lai Chia-Hsin; Liu Ching-Yuan;
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作者单位

Natl Cent Univ Dept Chem &

Mat Engn Taoyuan 320 Taiwan;

Chang Gung Univ Dept Pediat Chang Gung Mem Hosp Dept Chem &

Mat Engn Taoyuan 333 Taiwan;

Natl Cent Univ Dept Chem &

Mat Engn Taoyuan 320 Taiwan;

Natl Cent Univ Dept Chem &

Mat Engn Taoyuan 320 Taiwan;

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原文格式 PDF
正文语种 eng
中图分类化学;
关键词
arylation; C-H activation; energy conversion; hole-transporting materials; solar cells;

机译：芳基化;C-H激活;能量转换;孔输送材料;太阳能电池;

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1. Stable high-performance hybrid perovskite solar cells with ultrathin polythiophene as hole-transporting layer [J] . Weibo Yan1, Yunlong Li1, Yu Li2, 纳米研究：英文版 . 2015,第008期
2. The donor-dependent methoxy effects on the performance of hole-transporting materials for perovskite solar cells [J] . Mengyuan Li, Jinhua Wu, Guoguo Wang, 天然气化学（英文版） . 2020,第008期
3. The donor-dependent methoxy effects on the performance of hole-transporting materials for perovskite solar cells [J] . Mengyuan Li, Jinhua Wua, Guoguo Wang, 能源化学：英文版 . 2020,第008期
4. Direct C-H Arylation Meets Perovskite Solar Cells: Tin-Free Synthesis Shortcut to High-Performance Hole-Transporting Materials [J] . Chang Yu-Chieh, Lee Kun-Mu, Lai Chia-Hsin, Chemistry, an Asian journal . 2018,第11期

机译：直接C-H芳基化符合Perovskite太阳能电池：无酸合成快捷速度，高性能孔输送材料
5. Phenothiazine Functionalized Multifunctional A-pi-D-pi-D-pi-A-Type Hole-Transporting Materials via Sequential C-H Arylation Approach for Efficient and Stable Perovskite Solar Cells [J] . Lu Chunyuan, Paramasivam Mahalingavelar, Park Kyutai, ACS applied materials & interfaces . 2019,第15期

机译：吩噻嗪官能化多功能A-PI-D-PI-A型通过顺序C-H芳族化方法用于高效稳定的钙钛矿太阳能电池
6. Connecting Direct C-H Arylation Reactions with Dye-Sensitized Solar Cells: A Shortcut to D-A--A Organic Dyes [J] . Lin Po-Han, Lu Te-Jui, Cai Deng-Jhou, ChemSusChem . 2015,第19期

机译：用染料敏化太阳能电池连接直接C-H芳基化反应：D-A的快捷方式 - 有机染料
7. One-pot synthesis of D–p–D–p–D type holetransporting materials for perovskite solar cells by sequential C–H (hetero)arylations [C] . Chang-Chieh Ting, Kuan-Ming Lu, Kun-Mu Lee, 2019年第66回応用物理学会春季学術講演会講演予稿集 . 2019

机译：钙钛矿型太阳能电池的D–p–D–p–D型空穴传输材料通过连续C–H（杂）芳基化反应一锅合成
8. Development of Direct Arylation Polymerization Methodologies for Conjugated Copolymers and the Synthesis and Characterization of Indacenodithienothiophene Electron Accepting Molecules for Organic Solar Cells [D] . Aldrich, Thomas Jordan. 2019

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9. High-Performance Regular Perovskite Solar Cells Employing Low-Cost Poly(ethylenedioxythiophene) as a Hole-Transporting Material [O] . Xiaoqing Jiang, Ze Yu, Yuchen Zhang, -1

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10. Low-Cost, High-Performance Organic Small Molecular Hole-Transporting Materials for Perovskite Solar Cells [O] . Jiang-Yang Shao, Yu-Wu Zhong 2021

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11. Developing Efficient Charge-Selective Interfacial Materials for Polymer and Perovskite Solar Cells. [R] . Jen, A. K. 2016

机译：为聚合物和钙钛矿太阳能电池开发高效电荷选择性界面材料。

Direct C-H Arylation Meets Perovskite Solar Cells: Tin-Free Synthesis Shortcut to High-Performance Hole-Transporting Materials

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