Covalent Post-Assembly Modification: A Synthetic Multipurpose Tool in Supramolecular Chemistry

Zeng Haoxiang; Stewart-Yates Luke; Casey Louis M.; Bampos Nick; Roberts Derrick A.

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Covalent Post-Assembly Modification: A Synthetic Multipurpose Tool in Supramolecular Chemistry

机译：共价装配后修饰：超分子化学中的合成多功能工具

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摘要

The use of covalent post-assembly modification (PAM) in supramolecular chemistry has grown significantly in recent years, to the point where PAM is now a versatile synthesis tool for tuning, modulating, and expanding the functionality of self-assembled complexes and materials. PAM underpins supramolecular template-synthesis strategies, enables modular derivatization of supramolecular assemblies, permits the covalent 'locking' of unstable structures, and can trigger controlled structural transformations between different assembled morphologies. This Review discusses key examples of PAM spanning a range of material classes, including discrete supramolecular complexes, self-assembled soft nanostructures and hierarchically ordered polymeric and framework materials. As such, we hope to highlight how PAM has continued to evolve as a creative and functional addition to the synthetic chemist's toolbox for constructing bespoke self-assembled complexes and materials.

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来源
《ChemPlusChem》 |2020年第6期|共21页
作者
Zeng Haoxiang; Stewart-Yates Luke; Casey Louis M.; Bampos Nick; Roberts Derrick A.;
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作者单位

Univ Sydney Sch Chem Sydney NSW 2006 Australia;

Univ Sydney Sch Chem Sydney NSW 2006 Australia;

Univ Sydney Sch Chem Sydney NSW 2006 Australia;

Univ Sydney Key Ctr Polymers &

Colloids Sydney NSW 2006 Australia;

Univ Sydney Sch Chem Sydney NSW 2006 Australia;

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原文格式 PDF
正文语种 eng
中图分类化学;
关键词
coordination complexes; molecular self-assembly; post-synthetic modification; supramolecular chemistry; template synthesis;

机译：协调复合物;分子自组装;合成后修饰;超分子化学;模板合成;

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2. Covalent and Non-covalent Chemical Modification of Multi-walled Carbon Nanotubes with Tetra-（4-hydroxylphenyl）porphyrin and Its Complexes [J] . Zhao Hongbin, Wang Hongke, Chang Hui, 中国化学（英文版） . 2011,第009期
3. A simplified method for local tool interference detection and tool position modification during five-axis ball-end milling process [J] . JIANG Dong-dong, ZHANG Song, LI Bin-xun 重庆大学学报（英文版） . 2018,第004期
4. Supramolecular Polymer Networks with Enhanced Mechanical Properties:The Marriage of Covalent Polymer and Metallacycle [J] . Yue-Yue Zhang, Feng Chen, Yang Li, 中国化学（英文版） . 2021,第010期
5. Covalent post-assembly modification in metallosupramolecular chemistry [J] . Roberts Derrick A., Pilgrim Ben S., Nitschke Jonathan R. Chemical Society Reviews . 2018,第2期

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机译：SURMOFs的化学：官能团的层选择性安装和荧光显微镜探测的合成后的共价修饰
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10. Applying the tools of chemistry (mass spectrometry and covalent modification by small molecule reagents) to the detection of prions and the study of their structure [O] . Christopher J Silva 2014

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12. Supramolecular Organization Using a Synthetic Analogue of Biomineralization [R] . Bianconi, P. A. 1997

机译：使用生物矿化的合成类似物的超分子组织

Covalent Post-Assembly Modification: A Synthetic Multipurpose Tool in Supramolecular Chemistry

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