100th Anniversary of Macromolecular Science Viewpoint: The Role of Hydrophobicity in Polymer Phenomena

Jeffrey C.  Foster; Irem  Akar; Marcus C.  Grocott; Amanda K.  Pearce; Robert T.  Mathers; Rachel K.  O’Reilly

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100th Anniversary of Macromolecular Science Viewpoint: The Role of Hydrophobicity in Polymer Phenomena

机译：大分子科学观点100周年：疏水性在聚合物现象中的作用

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The seemingly simple notion of the hydrophobic effect can be viewed from multiple angles involving theory, simulation, and experiments. This viewpoint examines five attributes of predictive models to enhance synthetic efforts as well as experimental methods to quantify hydrophobicity. In addition, we compare existing predictive models against experimental data for polymer surface tension, lower critical solution temperature, solution self-assembly morphology, and degradation behavior. Key conclusions suggest that both the Hildebrand solubility parameters (HSPs) and surface area-normalized Log P (Log P SA~(–1)) values provide unique and complementary insights into polymer phenomena. In particular, HSPs appear to better describe bulk polymer phenomena for thermoplastics such as surface tension, while Log P SA~(–1) values are well-suited for describing and predicting the behavior of polymers in solution.

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《ACS Macro Letters》 |2020年第11期|共8页
作者
Jeffrey C. Foster; Irem Akar; Marcus C. Grocott; Amanda K. Pearce; Robert T. Mathers; Rachel K. O’Reilly;
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School of Chemistry University of Birmingham;

School of Chemistry University of Birmingham;

School of Chemistry University of Birmingham;

School of Chemistry University of Birmingham;

Department of Chemistry Pennsylvania State University;

School of Chemistry University of Birmingham;

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正文语种 eng
中图分类有机化学;
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100th Anniversary of Macromolecular Science Viewpoint: The Role of Hydrophobicity in Polymer Phenomena

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