Development of an Osmium Redox Polymer Mediated Bioanode and Examination of its Performance in        <i xmlns='http://www.wiley.com/namespaces/wiley'>Gluconobacter oxydansGluconobacter oxydans        Based Microbial Fuel Cell

Aslan Sema; Conghaile Peter ó; Leech Dónal; Gorton Lo; Timur Suna; Anik Ulku

摘要

Abstract > Gluconobacter oxydans ( G. oxydans ) cells together with an osmium redox polymer (ORP) [Osmium (2,2’‐bipyridine)2(poly‐vinylimidazole)10Cl]Cl were combined with a glassy carbon paste electrode (GCPE) to form a bioanode for a microbial fuel cell (MFC) based on G. oxydans . Although there are G.oxydans / ORP combined bioanode in the literature, as far as it is known, this system is the first one where G.oxydans /ORP bioanode is combined with a cathode and a MFC is formed. After the optimization of experimental parameters, analytical characteristics of ORP/ G. oxydans /GCPE bioanode were investigated. ORP/ G. oxydans /GCPE showed two linear ranges for ethanol substrate as 1.0–30?mM (R 2 =0.902) and 30–500?mM (R 2 =0.997) and analytical range as 1.0–1000?mM. Limit of detection (3.0?s/m) and limit of quantification (10?s/m) values were calculated as 1.29?mM and 4.30?mM respectively where the RSD value was 1.16?% for n=5. Combining the developed bioanode in the presence of 5.0?mM K <sub>3</sub> Fe(CN) <sub>6</sub> mediator with a Pt wire cathode a double compartment MFC was obtained via a salt bridge. G. oxydans /GCPE bioanode based MFC had maximum power density of 0.133 μW cm ?2 (at 33.5 mV), maximum current density as 8.73 μA cm ?2 and OCP value of 156 mV. On the other hand, ORP/ G. oxydans /GCPE based MFC showed maximum power density as 0.26 μW cm ?2 (at 46.8 mV), maximum current density as 15.079 μA cm ‐2 and OC </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span>None </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-22546/'>《Electroanalysis》</a> <b style="margin: 0 2px;">|</b><span>2017年第6期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Aslan Sema&option=202" target="_blank" rel="nofollow">Aslan Sema;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Conghaile Peter ó&option=202" target="_blank" rel="nofollow">Conghaile Peter ó;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Leech Dónal&option=202" target="_blank" rel="nofollow">Leech Dónal;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gorton Lo&option=202" target="_blank" rel="nofollow">Gorton Lo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Timur Suna&option=202" target="_blank" rel="nofollow">Timur Suna;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Anik Ulku&option=202" target="_blank" rel="nofollow">Anik Ulku;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Chemistry DepartmentMu?la S?tk? Ko?man University Faculty of Science48000 K?tekli/Mu?la Turkey;</p> <p>School of ChemistryNational University of Ireland GalwayUniversity Road Galway Ireland;</p> <p>School of ChemistryNational University of Ireland GalwayUniversity Road Galway Ireland;</p> <p>Department of Analytical Chemistry/Biochemistry and Structural BiologyLund UniversityPO Box 124 SE-22100 Lund Sweden;</p> <p>Faculty of ScienceEge University35100-Bornova Izmir Turkey;</p> <p>Chemistry DepartmentMu?la S?tk? Ko?man University Faculty of Science48000 K?tekli/Mu?la Turkey;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/4817.html" title="电化学、电解、磁化学">电化学、电解、磁化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=microbial biofuel cell&option=203" rel="nofollow">microbial biofuel cell;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=osmium redox polymer&option=203" rel="nofollow">osmium redox polymer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gluconobacter oxydans&option=203" rel="nofollow">Gluconobacter oxydans;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Glassy carbon paste electrodes&option=203" rel="nofollow">Glassy carbon paste electrodes;</a> </p> <div class="translation"> 机译：微生物生物燃料细胞;锇氧化还原聚合物;葡糖糖氧化物;玻璃碳浆料电极; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-harbin-institute-technology-new-series_thesis/0201234446869.html">Numerical Modeling of Microbial Fuel Cell Based on Redox Electron Mediator</a> <b>[J]</b> . <span> <a 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Development of an Osmium Redox Polymer Mediated Bioanode and Examination of its Performance in Gluconobacter oxydansGluconobacter oxydans Based Microbial Fuel Cell

摘要