Metal-Organic Frameworks as Heterogeneous Electrocatalysts for Water Splitting and CO2 Fixation

Zhang Peng-Feng; Wu Dan; Yang Guo-Ping; Wang Yao-Yu

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Metal-Organic Frameworks as Heterogeneous Electrocatalysts for Water Splitting and CO2 Fixation

机译：金属有机框架作为水分裂和CO2固定的异质电催化剂

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The reasonable design and preparation of cheap, Earth-abundant, efficient, and durable heterogeneous electrocatalytic materials are a probable solution to the key problems of energy shortages and environmental pollution. Metal-organic frameworks (MOFs) are widely utilized as heterogeneous electrocatalysts for the hydrogen evolution reaction (HER), oxygen evolution reaction (OER), overall water splitting, and carbon dioxide reduction reaction (CO2RR) owing to their high porosity, adjustable pore size/shape, redox characteristics, and other special structural features. This review generalizes the representative recent progress of MOFs as heterogeneous catalytic electrocatalysts for water splitting and the CO2RR and proposes strategies for devising MOF-based electrocatalytic catalysts for water splitting and the CO2RR. Finally, it summarizes the basic understanding and challenges of electrocatalysis on MOFs.

机译：合理设计和制备廉价、富土、高效、耐用的多相电催化材料是解决能源短缺和环境污染等关键问题的可能途径。金属有机骨架（MOF）由于其高孔隙率、可调节的孔径/形状、氧化还原特性和其他特殊结构特征，被广泛用作析氢反应（HER）、析氧反应（OER）、整体水分解和二氧化碳还原反应（CO2RR）的非均相电催化剂。本文综述了MOF作为多相催化电催化剂用于水分解和CO2RR的代表性最新进展，并提出了设计MOF基电催化剂用于水分解和CO2RR的策略。最后，总结了对MOFs电催化的基本认识和挑战。

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来源
《Crystal growth & design》 |2021年第6期|共20页
作者
Zhang Peng-Feng; Wu Dan; Yang Guo-Ping; Wang Yao-Yu;
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作者单位

Northwest Univ Coll Chem &

Mat Sci Key Lab Synthet &

Nat Funct Mol Minist Educ Shaanxi Key Lab Phys Inorgan Chem Xian 710127 Peoples R China;

Northwest Univ Coll Chem &

Mat Sci Key Lab Synthet &

Nat Funct Mol Minist Educ Shaanxi Key Lab Phys Inorgan Chem Xian 710127 Peoples R China;

Northwest Univ Coll Chem &

Mat Sci Key Lab Synthet &

Nat Funct Mol Minist Educ Shaanxi Key Lab Phys Inorgan Chem Xian 710127 Peoples R China;

Northwest Univ Coll Chem &

Mat Sci Key Lab Synthet &

Nat Funct Mol Minist Educ Shaanxi Key Lab Phys Inorgan Chem Xian 710127 Peoples R China;

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正文语种 eng
中图分类晶体学;
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1. Metal-organic framework derived Co3O4/PPy bifunctional electrocatalysts for efficient overall water splitting [J] . Yongli Tong, Hengqi Liu, Meizhen Dai, 中国化学快报（英文版） . 2020,第009期
2. Metal-organic framework derived CoSe2 nanoparticles anchored on carbon fibers as bifunctional electrocatalysts for efficient overall water splitting [J] . Chencheng, Sun1, Qiuchun, 纳米研究：英文版 . 2016,第008期
3. Metal-organic framework derived CoSe2 nanoparticles anchored on carbon fibers as bifunctional electrocatalysts for efficient overall water splitting [J] . Chencheng Sun, Qiuchun Dong, Jun Yang, 纳米研究（英文版） . 2016,第008期
4. Cable-like carbon nanotubes decorated metal-organic framework derived ultrathin CoSe2/CNTs nanosheets for electrocatalytic overall water splitting [J] . Guijuan Wei, Kun Du, Xixia Zhao, 中国化学快报（英文版） . 2020,第010期
5. Metal-organic framework coated titanium dioxide nanorod array p-n heterojunction photoanode for solar water-splitting [J] . Hui Yang1, Joeseph Bright1, Sujan Kasani4, 纳米研究：英文版 . 2019,第003期
6. Three-Dimensional N-Doped Carbon Nanotube Frameworks on Ni Foam Derived from a Metal-Organic Framework as a Bifunctional Electrocatalyst for Overall Water Splitting [J] . International journal of applied mechanics . 2020,第3期

机译：在Ni泡沫上衍生自金属有机框架的三维N掺杂碳纳米管框架作为整体水分裂的双官能电催化剂
7. Three-Dimensional N-Doped Carbon Nanotube Frameworks on Ni Foam Derived from a Metal-Organic Framework as a Bifunctional Electrocatalyst for Overall Water Splitting [J] . Yuan Qunyao, Yu Youxing, Gong Yongji, ACS applied materials & interfaces . 2020,第3期

机译：在Ni泡沫上衍生自金属有机框架的三维N掺杂碳纳米管框架作为整体水分裂的双官能电催化剂
8. Metal-organic framework derived CoTe2 encapsulated in nitrogen-doped carbon nanotube frameworks: a high-efficiency bifunctional electrocatalyst for overall water splitting [J] . Wang Xiang, Huang Xiaokang, Gao Wenbin, Journal of Materials Chemistry, A. Materials for energy and sustainability . 2018,第8期

机译：金属有机框架衍生的Cote2封装在氮气掺杂的碳纳米管框架中：用于整体水分裂的高效双官能电催化剂
9. Controlled Phase and Porosity of Cobalt Disulfide Nanoparticles through Metal-Organic Frameworks As Efficient Bifunctional Electrocatalysts for Overall Water Splitting [C] . In-Kyoung Ahn, Wonhyo Joo, Ji-Hoon Lee, Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

机译：通过金属 - 有机框架作为总水分分裂的高效双官能电催化剂的金属 - 有机框架对照相和孔隙率
10. FE-Doped Nickel Sulfide on Nickel Foam as Electrocatalyst for the Overall Splitting of Water [D] . Regalado Vera, Clarita Yosune 2019

机译：镍泡沫上富铁掺杂的硫化镍作为水总分解的电催化剂
11. Defect‐Rich Heterogeneous MoS2/NiS2 Nanosheets Electrocatalysts for Efficient Overall Water Splitting [O] . Jinghuang Lin, Pengcheng Wang, Haohan Wang, 2019

机译：富含缺陷的多相MoS2 / NiS2纳米片电催化剂可有效地进行总水分解
12. Metal-organic Framework-driven Porous Cobalt Disulfide Nanoparticles Fabricated by Gaseous Sulfurization as Bifunctional Electrocatalysts for Overall Water Splitting [O] . In-Kyoung Ahn, Wonhyo Joo, Ji-Hoon Lee, 2019

机译：金属 - 有机框架驱动的多孔钴二硫化物纳米硫化物，由气态硫化为整体水分裂的双官能电催化剂
13. Water Stabilization of Zr6-Based Metal-Organic Frameworks via Solvent-Assisted Ligand Incorporation. [R] . Deria, P., Chung, Y. G., Snurr, R. Q., 2015

机译：通过溶剂辅助配体加入Zr6基金属有机骨架的水稳定性。

Metal-Organic Frameworks as Heterogeneous Electrocatalysts for Water Splitting and CO2 Fixation

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