Analysis of the Growth of Laterally Aligned SnO2 Nanowires by Thermodynamic Considerations and Experiments

Jasmin-Clara  Bürger; Sebastian  Gutsch; Yi  Thomann; Ralf  Thomann; Bj?rn  Christian; Oliver  Ambacher; Margit  Zacharias

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Analysis of the Growth of Laterally Aligned SnO2 Nanowires by Thermodynamic Considerations and Experiments

机译：热力学考虑因素和实验分析横向对齐的SnO2纳米线的生长

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Recently, we reported the experimental tuning of the growth of freestanding SnO_(2) nanowires to a laterally aligned nanowire growth mode. Here, we present thermodynamic considerations taking into account the previously reported influencing parameters determining the experiments, i.e., the total pressure, the Sn/O ratio at the sample sites, the nanowire diameter, and the substrate type. We will discuss process parameters which will prefer a laterally aligned growth mode. We show that a continuous gold film used as catalyst inhibits the laterally aligned growth. Only at the edges the lateral growth can proceed, whereas the area region is covered by freestanding wires. The reason for that will be explained in a model. Furthermore, the laterally aligned nanowire surface faceting is analyzed by means of transmission electron microscopy and atomic force microscopy and explained.

机译：最近，我们报道了将独立式SnO_2纳米线的生长调整为横向排列的纳米线生长模式的实验。在这里，我们提出了热力学方面的考虑，其中考虑了之前报道的决定实验的影响参数，即总压、样品位置的Sn/O比、纳米线直径和衬底类型。我们将讨论更倾向于横向排列生长模式的工艺参数。我们发现，作为催化剂的连续金膜抑制了横向排列的生长。只有在边缘才能进行横向生长，而该区域由独立的导线覆盖。原因将在模型中解释。此外，利用透射电子显微镜和原子力显微镜对横向排列的纳米线表面刻面进行了分析和解释。

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《Crystal growth & design》 |2021年第1期|共9页
作者
Jasmin-Clara Bürger; Sebastian Gutsch; Yi Thomann; Ralf Thomann; Bj?rn Christian; Oliver Ambacher; Margit Zacharias;
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Laboratory for Nanotechnology Department of Microsystems Engineering (IMTEK) University of Freiburg;

Laboratory for Nanotechnology Department of Microsystems Engineering (IMTEK) University of Freiburg;

Freiburg Center for Interactive Materials and Bioinspired Technologies (FIT) University of Freiburg;

Freiburg Materials Research Center (FMF) and Institute for Macromolecular Chemistry University of Freiburg;

Department of Sustainable Systems Engineering (INATECH) University of Freiburg Emmy-Noether-Strasse;

Department of Sustainable Systems Engineering (INATECH) University of Freiburg Emmy-Noether-Strasse;

Laboratory for Nanotechnology Department of Microsystems Engineering (IMTEK) University of Freiburg;

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中图分类晶体学;
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1. Growth mechanism and photoluminescence of the SnO2 nanotwists on thin film and the SnO2 short nanowires on nanorods [J] . Wang Bing, Xu Ping 中国物理：英文版 . 2009,第001期
2. In-situ growth of vertically aligned nickel cobalt sulfide nanowires on carbon nanotube fibers for high capacitance all-solid-state asymmetric fiber-supercapacitors [J] . Na Liu, Zhenghui Pan, Xiaoyu Ding, 能源化学：英文版 . 2020,第002期
3. In-situ growth of vertically aligned nickel cobalt sulfide nanowires on carbon nanotube fibers for high capacitance all-solid-state asymmetric fiber-supercapacitors [J] . Na Liu, Zhenghui Pan, Xiaoyu Ding, 天然气化学（英文版） . 2020,第002期
4. Lateral epitaxial growth of faceted SnO2 nanowires with self-alignment [J] . Kim Won-Sik, Kim Daihong, Hong Seong-Hyeon CrystEngComm . 2014,第39期

机译：具有自对准的刻面SnO2纳米线的横向外延生长
5. Halide vapor phase epitaxy of ZnO studied by thermodynamic analysis and growth experiments [J] . Tetsuo Fujii, Naoki Yoshii, Yoshinao Kumagai, Journal of Crystal Growth . 2011,第1期

机译：热力学分析和生长实验研究ZnO的卤化物气相外延
6. A Thermodynamic Analysis of Microbial Growth Experiments [J] . JENNIFER N. SMITH, EVERETT L. SHOCK Astrobiology . 2007,第6期

机译：微生物生长实验的热力学分析
7. Effect of Growth Parameters on SnO2 Nanowires Growth by Electron Beam Evaporation Method [C] . R. Rakesh Kumar, Y. Manjula, K. Narasimha Rao International Conference on Advances in Materials and Manufacturing Applications . 2018

机译：电子束蒸发法生长参数对SnO2纳米线生长的影响
8. Novel approach to the growth and characterization of aligned epitaxial gallium nitride nanowires. [D] . Henry, Tania Alicia. 2010

机译：对准外延氮化镓纳米线的生长和表征的新颖方法。
9. Transition from freestanding SnO2 nanowires to laterally aligned nanowires with a simulation-based experimental design [O] . Jasmin-Clara Bürger, Sebastian Gutsch, Margit Zacharias 2020

机译：从独立式SnO2纳米线过渡到横向对齐的纳米线采用基于仿真的实验设计
10. Analysis of the Growth of Laterally Aligned SnO2 Nanowires by Thermodynamic Considerations and Experiments [O] . -1

机译：热力学考虑和实验对横向对齐的SnO2纳米线的生长分析
11. Growth of Vertically Aligned ZnO Nanowire Arrays Using Bilayered Metal Catalysts. [R] . E. R. Glaser H. Qi J. D. Caldwell S. M. Prokes 2012

机译：双层金属催化剂生长垂直排列的ZnO纳米线阵列。

Analysis of the Growth of Laterally Aligned SnO2 Nanowires by Thermodynamic Considerations and Experiments

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