Preparation of a modified g-C3N4 catalyst library and realization of a two-dimensional screening reaction

Liu Fenli; Bi Sifan; Wang Wenjing; Duan Qiannan; Feng Yunjin; Chen Jiayuan; Luo Run; Huang Yicai; Lee Jianchao

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Preparation of a modified g-C3N4 catalyst library and realization of a two-dimensional screening reaction

机译：改性G-C3N4催化剂文库的制备及二维筛选反应的实现

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In this study, we present a new fluorescence imaging-based high-throughput screening method to evaluate the catalytic performance of the polymetallic sulfide complex g-C3N4. In order to obtain a large number of catalysts, we chose the sulfates of three metals (Cd, Cu, and Ni) to modify g-C3N4. A catalyst library consisting of polymetallic sulfide composite carbon nitride materials (M3S/g-C3N4, M = CdxCuyNi1-x-y) was obtained using a color ink-jet printing technique. The degradation reaction of eosin solution was carried out under 365 nm UV light. According to the intensity of fluorescence change, the high-efficiency catalysts are the following three combinations: Cd0.37Cu0.53Ni0.10 S/g-C3N4, Cd0.11Cu0.41Ni0.48S/g-C3N4 and Cd0.31Cu0.39Ni0.30S/g-C3N4.

机译：在本研究中，我们提出了一种新的基于荧光成像的高通量筛选方法来评估多金属硫化物络合物g-C3N4的催化性能。为了获得大量的催化剂，我们选择了三种金属（镉、铜和镍）的硫酸盐来修饰g-C3N4。采用彩色喷墨打印技术获得了由多金属硫化物复合氮化碳材料（M3S/g-C3N4，M=CdxCuyNi1-x-y）组成的催化剂库。曙红溶液在365nm紫外光下进行降解反应。根据荧光强度的变化，高效催化剂有以下三种组合：Cd0。37Cu0。53Ni0。10 S/g-C3N4，Cd0。11Cu0。41Ni0。48S/g-C3N4和Cd0。31Cu0。39Ni0。30S/g-C3N4。

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《New Journal of Chemistry》 |2021年第5期|共7页
作者
Liu Fenli; Bi Sifan; Wang Wenjing; Duan Qiannan; Feng Yunjin; Chen Jiayuan; Luo Run; Huang Yicai; Lee Jianchao;
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Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Northwest Univ Coll Urban &

Environm Sci Shaanxi Key Lab Earth Surface Syst &

Environm Car Xian 710127 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

Shaanxi Normal Univ Sch Geog &

Tourism Dept Environm Sci Lab Env Mat Xian 710062 Peoples R China;

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正文语种 eng
中图分类化学;
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Preparation of a modified g-C3N4 catalyst library and realization of a two-dimensional screening reaction

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