A new zeolitic lithium aluminum imidazolate framework

Jiang Guangshen; Bon Volodymyr; Xu Fei; Garai Bikash; Zhang En; Senkovska Irena; Poetke Stephanie; Hippauf Felix; Hausdorf Steffen; Paasch Silvia; Brunner Eike; Wang Hongqiang; Kaskel Stefan

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A new zeolitic lithium aluminum imidazolate framework

机译：一种新的沸石锂铝咪唑酯框架

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An aliovalent mixed-metal framework DUT-174 [LiAl(2-methylimidazolate)(4)](n), isostructural to ZIF-8, was synthesized from lithium aluminum hydride (LiAlH4) and 2-methylimidazole (2-mImH) through dehydrogenation. Lithium and aluminum cations acting as alternating framework nodes are coordinated tetrahedrally by (2-mIm)(-). DUT-174 has a high specific surface area of 1149 m(2) g(-1) and CO2 uptake of 11.57 mmol g(-1) at 195 K.

机译：以锂铝氢化物（LiAlH4）和2-甲基咪唑（2-mImH）为原料，通过脱氢反应合成了与ZIF-8同构的异价混合金属骨架DUT-174[LiAl（2-甲基咪唑）（4）]（n）。作为交替骨架节点的锂和铝阳离子通过（2-mIm）（）四面体配位。DUT-174在195 K时具有1149 m（2）g（-1）的高比表面积和11.57 mmol g（-1）的CO2吸收。

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《Dalton transactions: An international journal of inorganic chemistry》 |2021年第23期|共5页
作者
Jiang Guangshen; Bon Volodymyr; Xu Fei; Garai Bikash; Zhang En; Senkovska Irena; Poetke Stephanie; Hippauf Felix; Hausdorf Steffen; Paasch Silvia; Brunner Eike; Wang Hongqiang; Kaskel Stefan;
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Northwestern Polytech Univ State Key Lab Solidificat Proc Sch Mat Sci &

Engn Shaanxi Joint Lab Graphene NPU Xian 710072 Peoples R China;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

Northwestern Polytech Univ State Key Lab Solidificat Proc Sch Mat Sci &

Engn Shaanxi Joint Lab Graphene NPU Xian 710072 Peoples R China;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

Fraunhofer Inst Mat &

Beam Technol IWS Winterbergstr 28 D-01277 Dresden Germany;

Fraunhofer Inst Mat &

Beam Technol IWS Winterbergstr 28 D-01277 Dresden Germany;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

Tech Univ Dresden Dept Bioanalyt Chem Bergstr 66 D-01062 Dresden Germany;

Tech Univ Dresden Dept Bioanalyt Chem Bergstr 66 D-01062 Dresden Germany;

Northwestern Polytech Univ State Key Lab Solidificat Proc Sch Mat Sci &

Engn Shaanxi Joint Lab Graphene NPU Xian 710072 Peoples R China;

Tech Univ Dresden Dept Inorgan Chem Bergstr 66 D-01062 Dresden Germany;

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正文语种 eng
中图分类化学;无机化学;
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A new zeolitic lithium aluminum imidazolate framework

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