1D Mn(iii) coordination polymers exhibiting chiral symmetry breaking and weak ferromagnetism

Hara Aoi; Kusumoto Sotaro; Sekine Yoshihiro; Harrowfield Jack; Kim Yang; Hayami Shinya; Nakamura Masaaki

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1D Mn(iii) coordination polymers exhibiting chiral symmetry breaking and weak ferromagnetism

机译：1D Mn（III）配位聚合物表现出手性对称性和弱铁磁性

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Mn(iii) complexes with achiral ligands, (E)-N-(2-((2-aminobenzylidene)amino)-2-methylpropyl)-5-X-2-hydroxybenzamide (HLX, X = H, Cl, Br, and I), crystallise as chiral conglomerates containing amide oxygen-bridged one-dimensional coordination polymers that exhibit weak ferromagnetism. The bulk products exhibit symmetry breaking in that they do not contain equal amounts of enantiomers, though which is the dominant species depends on the substituent X.

机译：Mn（iii）与非手性配体（E）-N-（2-（（2-氨基苄叉）氨基）-2-甲基丙基）-5-X-2-羟基苯甲酰胺（HLX，X=H，Cl，Br和I）的配合物结晶为含有酰胺氧桥联的一维配位聚合物的手性聚合物，表现出弱铁磁性。尽管占主导地位的物种取决于取代基X，但由于它们不包含等量的对映体，所以本体产物表现出对称性破缺。

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《Dalton transactions: An international journal of inorganic chemistry》 |2021年第16期|共5页
作者
Hara Aoi; Kusumoto Sotaro; Sekine Yoshihiro; Harrowfield Jack; Kim Yang; Hayami Shinya; Nakamura Masaaki;
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作者单位

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

Univ Strasbourg ISIS 8 Allee Gaspard Mange F-67083 Strasbourg France;

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

Kumamoto Univ Grad Sch Sci &

Technol Dept Chem Chuo Ku 2-39-1 Kurokami Kumamoto 8608555 Japan;

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正文语种 eng
中图分类化学;无机化学;
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2. Synthesis, structure, and magnetic properties of [Mn-III(salpn)NCS](n), a helical polymer, and the dimer [Mn-III(salpn)NCS](2). Weak ferromagnetism in [Mn-III(salpn)NCS](n) related to the strong magnetic anisotropy in Jahn-Teller Mn(III) (salpnH(2) N [J] . Sailaja S., Reddy KR., Rajasekharan MV., Inorganic Chemistry: A Research Journal that Includes Bioinorganic, Catalytic, Organometallic, Solid-State, and Synthetic Chemistry and Reaction Dynamics . 2003,第1期

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9. Chiral Symmetry and Chiral-Symmetry Breaking [R] . Peskin, M. E. 1982

机译：手性对称性与手性对称性破缺

1D Mn(iii) coordination polymers exhibiting chiral symmetry breaking and weak ferromagnetism

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