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One-pot transformation of polysaccharides via multi-catalytic processes

机译:通过多催化过程对多糖的一锅转化

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摘要

Much attention has been focused on the efficient transformations of renewable lignocellulosic biomass, particularly polysaccharides, to valuable chemicals and biofuels in the past decade. One strategy to produce chemicals from biomass in a more sustainable way is to integrate various types of catalytic process in a single pot. In contrast to multiple catalytic processes with separate reaction steps, the one-pot integration of sequential catalytic processes can maximize efficiency, minimize waste and increase profitability in the multistep transformation of biomass. The present article aims to review recent research progress towards the reasonable integration of sequential catalytic processes, to achieve the end goal of comprehensive utilization of biomass in both the chemical industry and academia. The systems described in this article mainly involve those using polysaccharides as the substrates and the coupling of different chemical/biological reactions in a single pot.
机译:在过去的十年中,人们关注了可再生木质纤维素生物量(尤其是多糖)对有价值的化学物质和生物燃料的有效转化。 以更可持续的方式从生物质中产生化学物质的一种策略是将各种类型的催化过程整合到一个锅中。 与具有单独的反应步骤的多个催化过程相反,顺序催化过程的一锅整合可以最大程度地提高效率,最大程度地减少废物并提高生物量多步化转化的利润率。 本文旨在回顾最新的研究进展,以合理地整合顺序的催化过程,以实现化学工业和学术界全面利用生物质的最终目标。 本文描述的系统主要涉及使用多糖作为底物和单个锅中不同化学/生物反应的偶联的系统。

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