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首页> 外文期刊>Catalysis science & technology >Controlling 1T/2H heterophase junctions in the MoS2 microsphere for the highly efficient photocatalytic hydrogen evolution
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Controlling 1T/2H heterophase junctions in the MoS2 microsphere for the highly efficient photocatalytic hydrogen evolution

机译:控制1 t / 2 h多相的连接二硫化钼高效的微球光催化氢进化

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摘要

The 1T/2H heterophase junction MoS2 2D nanolayer for assembly into microspheres were fabricated through a simple one-step hydrothermal synthesis. These unique junction structure MoS2 microspheres facilitate the separation of the electron-hole between different phases for forming the built-in electric field in the nanolayer. The content of 1T/2H heterophase junctions could be effectively regulated by simple changing the molar ratio of the Mo/S source in the synthesis processes. The prepared MoS2 microspheres as a photocatalyst enable the effective hydrogen production from water. The hydrogen production activity of the photocatalyst is dependent on the content of the heterophase junctions. The hydrogen production rate was the highest up to 22.4 mu mol h(-1) on the optimal sample MS (1 : 2).
机译:1吨/ 2 h多相结二硫化钼2 d nanolayer组装成微球是捏造的通过一个简单的一步水热合成。这些独特的二硫化钼微球结结构促进电子空穴的分离内置的不同阶段之间形成nanolayer电场。1吨/ 2 h多相连接可能是有效的由简单的摩尔比率的变化Mo / S源的合成过程。准备二硫化钼微球作为光催化剂使有效的制氢水。光催化剂是依赖的内容多相连接。率最高的22.4亩摩尔h (1)最优样本女士(1:2)。

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