Recent advances of the nano-hierarchical SAPO-34 in the methanol-to-olefin (MTO) reaction and other applications

Zhong Jiawei; Han Jingfeng; Wei YingxuTian PengGuo XinwenSong ChunshanLiu Zhongmin

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Recent advances of the nano-hierarchical SAPO-34 in the methanol-to-olefin (MTO) reaction and other applications

机译：最新进展的nano-hierarchical SAPO-34methanol-to-olefin (MTO)和反应其他应用程序

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摘要

The recent advances in synthesis and catalytic applications of nano-hierarchical SAPO-34 for methanol-to-olefin (MTO) conversion and other reactions have been elaborated in this minireview. The structure, unique properties (e.g., shape selectivity), and diffusion of zeolites and molecular sieves are briefly covered in the first part. An overview of the development of synthetic methods for the preparation of nanosized SAPO-34 and hierarchical SAPO-34 is included in the second and third parts, with focus on the novel and green preparation strategies. The advantages and disadvantages of the different synthetic approaches are discussed in detail, and the relationship between the catalytic performance and the diffusion and acidity is also elucidated. Finally, the updated characterization techniques considering the interconnectivity between the pore channels are outlined.

机译：合成和催化的最新进展应用nano-hierarchical SAPO-34和其他methanol-to-olefin (MTO)转换反应已经阐述了摘要概述。(例如,形状选择性)和扩散沸石分子筛是简要介绍在第一部分。的合成制备方法纳米SAPO-34和分层SAPO-34包含在第二和第三部分,专注于小说和绿色的准备策略。不同的合成方法进行了讨论在细节,和之间的关系催化性能和扩散酸度也阐明。表征技术考虑孔隙通道之间的互连概述了。

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来源
《Catalysis science & technology》 |2017年第21期|4905-4923|共19页
作者
Zhong Jiawei; Han Jingfeng; Wei YingxuTian PengGuo XinwenSong ChunshanLiu Zhongmin;
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作者单位

Chinese Acad Sci, State Energy Low Carbon Catalysis & Engn R&D Ctr, Natl Engn Lab Methanol Olefins,Dalian Inst Chem P, Dalian Natl Lab Clean Energy iChEM Collaborat Inn, Dalian 116023, Peoples R China;

Dalian Univ Technol, State Key Lab Fine Chem, PSU DUT Joint Ctr Energy Res, Sch Chem Engn, Dalian 116024, Peoples R China;

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正文语种英语
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关键词
Catalysis; SYNTHETICS; AcidityZeolitesMOLECULAR SIEVESREACTION;

机译：催化;合成材料;AcidityZeolitesMOLECULARSIEVESREACTION;

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专利

1. Kinetics of steam regeneration of SAPO-34 zeolite catalyst in methanol-to-olefins (MTO) process [J] . Huaiqing An, Hua Li, Jibin Zhou, 中国化学工程学报（英文版） . 2021,第007期
2. Performance of Methanol-to-Olefins Catalytic Reactions by the Addition of PEG in the Synthesis of SAPO-34 [J] . Yaquan Wang, Zhao Wang, Chao Sun, 天津大学学报（英文版） . 2017,第006期
3. An effective route to improve the catalytic performance of SAPO-34 in the methanol-to-olefin reaction [J] . Guangyu Liu, Peng Tian, Qinhua Xia, 天然气化学（英文版） . 2012,第004期
4. The template-assisted zinc ion incorporation in SAPO-34 and the enhanced ethylene selectivity in MTO reaction [J] . Jiawei Zhong, Jingfeng Han, Yingxu Wei, 能源化学：英文版 . 2019,第005期
5. The template-assisted zinc ion incorporation in SAPO-34 and the enhanced ethylene selectivity in MTO reaction [J] . Jiawei Zhong, Jingfeng Han, Yingxu Wei, 天然气化学（英文版） . 2019,第005期
6. A low-temperature approach to synthesize low-silica SAPO-34 nanocrystals and their application in the methanol-to-olefins (MTO) reaction [J] . Gao Beibei, Yang Miao, Qiao YuyanLi JinzheXiang XiaoWu PengfeiWei YingxuXu ShutaoTian PengLiu Zhongmin Catalysis science & technology . 2016,第20期

机译：低温合成方法二氧化硅SAPO-34纳米晶体和他们应用程序在methanol-to-olefins (MTO)反应
7. Improving the catalytic performance of SAPO-18 for the methanol-to-olefins (MTO) reaction by controlling the Si distribution and crystal size [J] . Martinez-Franco Raquel, Li Zhibin, Martinez-Triguero JoaquinMoliner ManuelCorma Avelino Catalysis science & technology . 2016,第8期

机译：改善SAPO-18的催化性能methanol-to-olefins (MTO)反应控制硅分布和晶粒大小
8. The Weight Change of SAPO-34 Catalyst During MTO Process in TGA Reactor [C] . Hao Hu, Weiyong Ying, Fahai Cao, International Materials Research Congress . 2010

机译：TGA反应器MTO过程中SAPO-34催化剂的重量变化
9. Tip-Enhanced Raman Spectroscopy Advances and Its Applications =针尖增强拉曼光谱的应用与进展 [D] . You, Xiao. 2019

机译：Tip-Enhanced Raman Spectroscopy Advances and Its Applications =针尖增强拉曼光谱的应用与进展
10. Nanosize-Enhanced Lifetime of SAPO-34 Catalysts in Methanol-to-Olefin Reactions [O] . Yang Guoju, Wei Yingxu, Xu Shutao, 2013

机译：Nanosize-Enhanced Lifetime of sapO-34 Catalysts in methanol-to-Olefin Reactions

Recent advances of the nano-hierarchical SAPO-34 in the methanol-to-olefin (MTO) reaction and other applications

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