Visible light promoted photocatalytic water oxidation: proton and electron collection via a reversible redox dye mediator

Walsh Dominic; Sanchez-Ballester Noelia M.; Ting Valeska P.Ariga KatsuhikoWeller Mark T.

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Visible light promoted photocatalytic water oxidation: proton and electron collection via a reversible redox dye mediator

机译：可见光促进光催化水氧化:质子和电子通过一个集合可逆的氧化还原染料中介

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Visible light promoted photocatalytic water oxidations were conducted using a homogenous cobalt complex as a catalyst that was absorbed onto a silica gel substrate. The porous SiO2 contained Ru(bpy)(3)(2+) as a light harvester and the redox quinone analogue DCPIP as a reversible electron mediator as a step towards utilization of protons and electrons liberated in water oxidations for solar fuels.

机译：可见光促进光催化水使用一个同质的氧化反应进行复杂钴作为催化剂,吸收到一个硅胶基质。包含俄文(bpy)(3)(2 +)作为光收割机作为一个可逆的氧化还原醌模拟DCPIP电子中介作为一步利用率质子和电子的解放在水里太阳能燃料氧化反应。

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《Catalysis science & technology》 |2016年第11期|3718-3722|共5页
作者
Walsh Dominic; Sanchez-Ballester Noelia M.; Ting Valeska P.Ariga KatsuhikoWeller Mark T.;
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作者单位

Univ Bath, Dept Chem, Claverton Down, Bath BA2 7AY, Avon, England;

Univ Strasbourg, Inst Charles Sadron, 23 Rue Loess,BP 84047, F-67034 Strasbourg, France;

Natl Inst Mat Sci, 1-2-1 Sengen, Tsukuba, Ibaraki 3050047, JapanUniv Bath, Dept Chem Engn, Bath BA2 7AY, Avon, England;

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正文语种英语
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关键词
oxidation reduction potential; Oxidation; electron collectionStepsVisible LightCOBALT COMPLEXESCatalystsMediator Complexhydrogen ionsRedox processes;

机译：氧化还原电位;氧化;电子collectionStepsVisible LightCOBALTCOMPLEXESCatalystsMediator ComplexhydrogenionsRedox流程;

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Visible light promoted photocatalytic water oxidation: proton and electron collection via a reversible redox dye mediator

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