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CO_2 Capture in Metal-Organic Framework Adsorbents: An Engineering Perspective

机译：二氧化碳捕获在有机框架吸附剂:一个工程的角度

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摘要

CO_2 emission has raised worldwide concerns because of its potential effects on climate change, species extinction, and plant nutrition deterioration. Metal-organic frameworks (MOFs) are one class of crystalline adsorbent materials that are believed to be of huge potential in CO_2 capture applications because of their advantages such as ultrahigh porosity, boundless chemical tunability, and surface functionality over traditional porous zeolites and activated carbon. In terms of chemistry, there are already many studies devoted to the synthesis of new functional MOFs. Some of the synthesized MOFs have been evaluated for CO2 capture at laboratory-scale. Several reviews have been published on this topic, but mainly from a chemistry and materials pointof view. In this review, the authors focus on the engineering perspective on this topic, with emphases on material evaluation, performance judgment, and process design to address the engineering issues of these materials to be used as adsorbents in industrial CO2 capture. The current engineering evaluation approaches for MOFs are summarized, in a manner that could also be applied to other adsorbent materials.
机译：二氧化碳排放引起了全球关注因为它的潜在影响气候变化,物种灭绝,和植物营养恶化。是一类结晶吸附剂材料这被认为是技术的巨大潜力捕获应用程序,因为他们的优势如超高孔隙度、无限的化学可调谐性和表面功能传统的多孔沸石和活性炭。在化学方面,已经有很多研究致力于合成新的功能性mof。已经评估了二氧化碳捕获实验室规模。发表关于这个主题,但主要来自一个化学和材料心态。审查,作者重点工程对这个话题的看法,重点材料评估、性能判断,流程设计来解决工程问题这些材料作为吸附剂工业二氧化碳捕获。财政部的评价方法进行了总结,在也可以应用于其他的方式吸附剂材料。

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