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Photochemical Systems for Solar-to-Fuel Production

机译:用于太阳能燃料生产的光化学系统

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The photochemical system,which utilizes only solar energy and H2O/CO2 to produce hydrogen/carbon-based fuels,is considered a promising approach to reduce CO2 emissions and achieve the goal of carbon neutrality.To date,numerous photochemical systems have been developed to obtain a viable solar-to-fuel production system with sufficient energy efficiency However,more effort is still needed to meet the requirements of industrial implementation.In this review,we systematically discuss a typical photochemical system for solar-to-fuel production,from classical theories and fundamental mechanisms to raw material selection,reaction condition optimization,and unit device/system advancement,from the viewpoint of ordered energy conversion.State-of-the-art photochemical systems,including photocatalytic,photovoltaic-electrochemical,photo-electrochemical,solar thermochemical,and other emerging systems,are summarized.We highlight the existing bottlenecks and discuss the developing trend of this technology.Finally,optimization strategies and new opportunities are proposed to enhance photochemical systems with higher energy efficiency.
机译:光化学系统,利用太阳能能源和水/二氧化碳来生产氢/碳基燃料,被认为是有前途的方法来减少二氧化碳排放实现碳中和的目标。日期,无数光化学系统发达国家获得一个可行的solar-to-fuel生产系统提供足够的能量然而,效率仍然需要更多的努力满足工业的需求实现。讨论一个典型的光化学系统solar-to-fuel生产,从经典理论和基本原材料的机制选择,反应条件优化和单位设备/系统的进步,从观点的能量转换。光化学系统,包括

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