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Recent advances in reducible metal oxide catalysts for C1 reactions

机译:用于C1反应的可还原金属氧化物催化剂的研究进展

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摘要

Chemical conversion of one-carbon (C1) molecules to value-added chemicals and energy fuels has attracted increasing research interest in recent years driven by concerns on the depletion of fossil fuel resources and amplifying environmental issues caused by anthropogenic activities. In this mini-review, we introduce important C1 reactions in CO, CO2, and CH4 conversions via different approaches, including thermally, electrochemically, and photochemically driven processes, and the catalysis mechanism of reducible metal oxide (RMO) materials for use in these reactions. We mainly summarize the latest research advances in RMO catalyst materials and their common functionality in these C1 reactions, discuss the current research status and challenges, and provide a perspective on future research directions and opportunities in this field.
机译:一个碳的化学转化(C1)分子增值的化学物质和能源燃料最近吸引了越来越多的研究兴趣年由枯竭的担忧化石燃料资源和放大人为造成的环境问题活动。重要C1反应CO、CO2和CH4通过不同的方法转换,包括热、电化学、光化学地驱动过程和催化机理可还原的金属氧化物(RMO)材料使用这些反应。研究进展在RMO材料和催化剂他们共同的功能在这些C1的反应,当前的研究现状和讨论未来的挑战,并提供一个视角研究方向和机会字段。

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