Preferential population of Al atoms at the T4 site of ZSM-35 for the carbonylation of dimethyl ether

Zhiping Xiong; Guodong Qi; Luyi Bai

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Preferential population of Al atoms at the T4 site of ZSM-35 for the carbonylation of dimethyl ether

机译：Preferential population of Al atoms at the T4 site of ZSM-35 for the carbonylation of dimethyl ether

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摘要

Hydrothermal synthesis of ZSM-35 using dioxane as the structure-directing agent resulted in more than half of Al atoms located at the T4 site in the 8 membered-ring pore.The Bronsted acid site,thus generated,efficiently catalyzed the carbonylation of dimethyl ether with a specific activity of 1.2 mol_(MA)mol_(T4)~(-1)h~(-1)at 493 K.

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《Catalysis science & technology》 |2022年第16期|4993-4997|共5页
作者
Zhiping Xiong; Guodong Qi; Luyi Bai;
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作者单位

State Key Laboratory of Catalysis,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian,China;

National Centre for Magnetic Resonance in Wuhan,State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics,Innovation Academy for Precision Measurement Science and Technology,Chinese Academy of Sciences,Wuhan,China;

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正文语种英语
中图分类物理化学（理论化学）、化学物理学;
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Preferential population of Al atoms at the T4 site of ZSM-35 for the carbonylation of dimethyl ether

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