Tethering Organic Disulfides to Layered Silicates: A Versatile Strategy for Photo-Controllable Dynamic Chemistry and Functionalization

Tanks Jonathon; Hiroi Takashi; Tamura KenjiNaito Kimiyoshi

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Tethering Organic Disulfides to Layered Silicates: A Versatile Strategy for Photo-Controllable Dynamic Chemistry and Functionalization

机译：Tethering Organic Disulfides to Layered Silicates: A Versatile Strategy for Photo-Controllable Dynamic Chemistry and Functionalization

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摘要

The dynamic covalent chemistry of molecular disulfides has been studied extensively in solution, but their reactivity when confined to nanospaces has not been investigated, nor has their application to functional nanomaterials been explored. In this study, symmetrical organic disulfides were tethered to the basal planes of synthetic mica by intercalation, confining photo -induced reactions to the interlayer as a result. This approach functionalizes the nanosheets to act as host for photo -induced disulfide-disulfide, disulfide-thiol, and disulfide-ene reactions, providing control and versatility for a wide variety of applications.

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来源
《Bulletin of the Chemical Society of Japan》 |2023年第1期|65-71|共7页
作者
Tanks Jonathon; Hiroi Takashi; Tamura KenjiNaito Kimiyoshi;
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作者单位

Tohoku Univ;

Natl Inst Mat Sci NIMS;

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原文格式 PDF
正文语种英语
中图分类化学;
关键词
Disulfide chemistry; Layered silicates; Photo-reactivity; COVALENT CHEMISTRY; THIOL; INTERCALATION; SURFACE;

Tethering Organic Disulfides to Layered Silicates: A Versatile Strategy for Photo-Controllable Dynamic Chemistry and Functionalization

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