A Low-Power CuSCN Hydrogen Sensor Operating Reversibly at Room Temperature

Kabitakis Viktoras; Gagaoudakis Emmanouil; Moschogiannaki MarilenaKiriakidis GeorgeSeitkhan AkmaralFirdaus YuliarFaber HendrikYengel EmreLoganathan KalaivananDeligeorgis GeorgeTsetseris LeonidasAnthopoulos Thomas D.Binas Vassilios

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A Low-Power CuSCN Hydrogen Sensor Operating Reversibly at Room Temperature

机译：A Low-Power CuSCN Hydrogen Sensor Operating Reversibly at Room Temperature

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Hydrogen is attractive as an abundant source for clean and renewable energy. However, due to its highly flammable nature in a range of concentrations, the need for reliable and sensitive sensor/monitoring technologies has become acute. Here a solid-state hydrogen sensor based on solution-processable p-type semiconductor copper thiocyanate (CuSCN) is developed and studied. Sensors incorporating interdigitated electrodes made of noble metals (gold, platinum, palladium) show excellent response to hydrogen concentration down to 200 ppm while simultaneously being able to operate reversibly at room temperature and at low power. Sensors incorporating Pd electrodes show the highest signal response of 179% with a response time of approximate to 400 s upon exposure to 1000 ppm of hydrogen gas. The experimental findings are corroborated by density functional theory calculations, which highlight the role of atomic hydrogen species created upon interaction with the noble metal electrode as the origin for the increased p-type conductivity of CuSCN during exposure. The work highlights CuSCN as a promising sensing element for low-power, all-solid-state printed hydrogen sensors.

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《Advanced functional materials》 |2022年第7期|2102635.1-2102635.9|共9页
作者
Kabitakis Viktoras; Gagaoudakis Emmanouil; Moschogiannaki MarilenaKiriakidis GeorgeSeitkhan AkmaralFirdaus YuliarFaber HendrikYengel EmreLoganathan KalaivananDeligeorgis GeorgeTsetseris LeonidasAnthopoulos Thomas D.Binas Vassilios;
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Fdn Res & Technol Hellas FORTH IESL, Inst Elect Struct & Laser, GR-71110 Iraklion, Greece;

King Abdullah Univ Sci & Technol KAUST, Phys Sci & Engn Div PSE, KAUST Solar Ctr KSC, Thuwal 239556900, Saudi Arabia;

King Abdullah Univ Sci & Technol KAUST, Phys Sci & Engn Div PSE, KAUST Solar Ctr KSC, Thuwal 239556900, Saudi Arabia|Natl Res & Innovat Agcy, Res Ctr Elect & Telecommun, Jalan Sangkuriang Komplek LIPI Bldg 20 Level 4, Bandung 40135, IndonesiaNatl Tech Univ Athens, Dept Phys, GR-15780 Athens, GreeceFdn Res & Technol Hellas FORTH IESL, Inst Elect Struct & Laser, GR-71110 Iraklion, Greece|Univ Crete, Dept Phys, GR-71110 Iraklion, Greece;

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copper (I) thiocyanate; hydrogen sensors; solution processable semiconductors;

A Low-Power CuSCN Hydrogen Sensor Operating Reversibly at Room Temperature

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