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A Multiscale Porous 3D-Fabric Evaporator with Vertically Aligned Yarns Enables Ultra-Efficient and Continuous Water Desalination

机译:A Multiscale Porous 3D-Fabric Evaporator with Vertically Aligned Yarns Enables Ultra-Efficient and Continuous Water Desalination

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摘要

Solar steam generation has emerged as an environment-friendly and promisingstrategy to overcome the freshwater and energy crisis. However,simultaneously attaining the satisfied evaporation rate, durability and energyutilization in a single system is challengeable, but crucial to the practicalapplication. Herein, inspired by the carpet weaving technique and benefitingfrom “fiber–yarn–fabric” hierarchical structures, a 3D fabric evaporator withvertical hemp-yarn arrays is innovatively constructed, featuring a combinedstructure of multiscale pores from tunable spacing between adjacent fibers oryarns, the vertically aligned architecture coated with superhydrophilic MXenesandwichedlayer and the adjustable side height/areas. These structures workcooperatively, surprisingly achieving the integrated functions of excellent lightcapture, the balanced evaporation area and vapor escape space, the additionalenergy adsorption from the environment and the salt exchange alongor between micro/macro pores. Consequently, the 3D evaporator exhibits anoutstanding evaporation rate (3.95 kg m~(?2) h~(?1) under one-sun illumination) andextremely high outdoor evaporation (47.04 kg m~(?2) for 8 h), accompanied withoutstanding salt-resistance (continuous 120 h in 14% brine without salt accumulation),anti-oilfouling and anti-bacterial (efficiency over 99.9%) performances.Finally, through rationally assembling multi-function modules with acondenser, an all-in-one “desalination–thermoelectricity–irrigation” platformis built, realizing the maximum utilization of steam condensation enthalpy.

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