Multi-Sites Electrocatalysis in High-Entropy Alloys

Li Hongdong; Lai Jianping; Li ZhenjiangWang Lei

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Multi-Sites Electrocatalysis in High-Entropy Alloys

机译：Multi-Sites Electrocatalysis in High-Entropy Alloys

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High-entropy alloys (HEAs) have attracted widespread attention in electrocatalysis due to their unique advantages (adjustable composition, complex surface, high tolerance, etc.). They allow for the formation of new and tailorable active sites in multiple elements adjacent to each other, and the interaction can be tailored by rational selection of element configuration and composition. However, it needs to be further explored in catalyst design, the interaction of elements, and the determination of active sites. This review article focuses on the important progress for multi-sites electrocatalysis in HEAs. The classification is done on the basis of catalytic reaction, including hydrogen evolution reaction, oxygen evolution reaction, oxygen reduction reaction, alcohol oxidation reaction, carbon dioxide reduction reaction, and nitrogen reduction reaction. Based on experiments and theories, a more in-depth exploration of the high catalytic activity of HEAs will be conducted, including the selection of elements (the special role of each element in catalysis) and the multi-sites effect. This review can provide the basis for the element selection and design of HEAs in some reactions, to adjust the compositions of HEAs to improve their intrinsic activity. Furthermore, the remaining challenges and future directions for promising research fields are also provided.

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《Advanced functional materials》 |2021年第47期|2106715.1-2106715.28|共28页
作者
Li Hongdong; Lai Jianping; Li ZhenjiangWang Lei;
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作者单位

Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Taishan Scholar Adv & Characterist Discipline Tea, Key Lab Ecochem Engn, Qingdao 266042, Peoples R China;

Qingdao Univ Sci & Technol, Coll Mat Sci & Engn, Qingdao 266042, Peoples R China;

Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Taishan Scholar Adv & Characterist Discipline Tea, Key Lab Ecochem Engn, Qingdao 266042, Peoples R China|Qingdao Univ Sci & Technol, Coll Environm & Safety Engn, Shandong Engn Res Ctr Marine Environm Corro;

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正文语种英语
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electrocatalysis; high-entropy alloys; multi-sites;

Multi-Sites Electrocatalysis in High-Entropy Alloys

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