Insights into Heterogeneous Catalysts under Reaction Conditions by In Situ/Operando Electron Microscopy

Han-Wen Cheng; Shan Wang; Guanyu ChenZhengwang LiuDominic CaraccioloMerry MadiouShiyao ShanJincang ZhangHeyong HeRenchao CheChuan-Jian Zhong

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Insights into Heterogeneous Catalysts under Reaction Conditions by In Situ/Operando Electron Microscopy

机译：Insights into Heterogeneous Catalysts under Reaction Conditions by In Situ/Operando Electron Microscopy

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The advancement of clean energy and environment depends strongly on thedevelopment of efficient catalysts in a wide range of heterogeneous catalyticreactions, which has benefited from transmission electron microscopictechniques in determining the atomic-scale morphologies and structures.However, it is the morphology and structure under the catalytic reaction conditionsthat determine the performance of the catalyst, which has captured asurge of interest in developing and applying in situ/operando transmissionelectron microscopic techniques in heterogeneous catalysis. The major themeof this review is to highlight some of the most recent insights into heterogeneouscatalysts under the relevant reaction conditions using in situ/operandotransmission electron microscopic techniques. Rather than a comprehensiveoverview of the basic principles of in situ/operando techniques, this reviewfocuses on the insights into the atomic-scale/nanoscale details of variouscatalysts ranging from single-component to multicomponent catalystsunder heterogeneous catalytic, electrocatalytic, and photocatalytic reactionconditions involving both gas–solid and liquid–solid interfaces. This focus iscoupled with discussions of the correlation of the atomic, molecular, andnanoscale morphology, composition, and structure with the catalytic propertiesunder the reaction conditions, shining light on the challenges andopportunities in design of nanostructured catalysts for clean and sustainableenergy applications.

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来源
《Advanced energy materials》 |2022年第38期|2202097.1-2202097.43|共43页
作者
Han-Wen Cheng; Shan Wang; Guanyu ChenZhengwang LiuDominic CaraccioloMerry MadiouShiyao ShanJincang ZhangHeyong HeRenchao CheChuan-Jian Zhong;
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作者单位

Laboratory of Advanced MaterialsShanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438, P. R. China;

Department of ChemistryState University of New York at BinghamtonBinghamton, NY 13902, USA;

Zhejiang LaboratoryHangzhou 311100, ChinaLaboratory of Advanced MaterialsShanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438, P. R. China Zhejiang LaboratoryHangzhou 311100, ChinaLaboratory of Advanced MaterialsShanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438, P. R. China Department of ChemistryState University of New York at BinghamtonBinghamton, NY 139;

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catalytic reactions; electrocatalytic reactions; heterogeneous catalysts; in situ/operando; transmission electron microscopy;

Insights into Heterogeneous Catalysts under Reaction Conditions by In Situ/Operando Electron Microscopy

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