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High Performing Solid-State Organic Electrochemical Transistors Enabled by Glycolated Polythiophene and Ion-Gel Electrolyte with a Wide Operation Temperature Range from ?50 to 110 ℃

机译:High Performing Solid-State Organic Electrochemical Transistors Enabled by Glycolated Polythiophene and Ion-Gel Electrolyte with a Wide Operation Temperature Range from ?50 to 110 ℃

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摘要

The development of organic electrochemical transistors (OECTs) capable ofmaintaining their high amplification, fast transient speed, and operationalstability in harsh environments will advance the growth of next-generationwearable and biological electronics. In this study, a high-performance solidstateOECT (SSOECT) is successfully demonstrated, showing a recorded hightransconductance of 220 ± 59 S cm~(?1), ultrafast device speed of ≈10 kHz withexcellent operational stability over 10 000 switching cycles, and thermallystable under a wide temperature range from ?50 to 110 ℃. The developedSSOECTs are successfully used to detect low-amplitude physiological signals,showing a high signal-to-noise-ratio of 32.5 ± 2.1 dB. For the first time, theamplifying power of these SSOECTs is also retained and reliably shown to collecthigh-quality electrophysiological signals even under harsh temperatures(?50 and 110 ℃). The demonstration of high-performing SSOECTs and itsapplication in harsh environment are core steps toward their implementationin next-generation wearable electronics and bioelectronics.

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