Research progress in stable interfacial constructions between composite polymer electrolytes and electrodes

Pan Jun; Zhao Pei; Wang NanaHuang FuqiangDou Shixue

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Research progress in stable interfacial constructions between composite polymer electrolytes and electrodes

机译：Research progress in stable interfacial constructions between composite polymer electrolytes and electrodes

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Composite polymer electrolytes (CPEs) have great commercialization potential because they can take advantage of the properties of inorganic and polymer electrolytes, which enable them to realize relatively high ionic conductivity, better electrode contacts, and superior mechanical strength. Nevertheless, the interface between the CPE and the electrode material remains a key challenge that obstructs the further practical development of polymer solid-state lithium batteries (PSSBs). This is because the continuous side reactions between the electrode materials and the CPE can result in unstable interfaces during cycling, thus affecting the electrochemical performance of the battery. Here, in this review, recent advances in various interfacial constructions are reviewed, including the modification of electrode materials and optimization of CPEs. Furthermore, we specifically focus on the underlying mechanisms of the interfacial contact, ionic migration, and electrochemical reactions between the electrodes and the CPE. It is hoped that this review can stimulate greater progress towards an in-depth understanding of this interfacial issue for CPEs, which could provide specific solutions for improving the electrochemical performances of PSSBs.

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来源
《Energy & environmental science: EES》 |2022年第7期|2753-2775|共23页
作者
Pan Jun; Zhao Pei; Wang NanaHuang FuqiangDou Shixue;
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作者单位

Univ Wollongong, Inst Superconducting & Elect Mat, Innovat Campus,Squires Way, Wollongong, NSW 2500, Australia;

Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China;

Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China|Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China;

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Research progress in stable interfacial constructions between composite polymer electrolytes and electrodes

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