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首页> 外文期刊>The Journal of Chemical Physics >Dissociation slowdown by collective optical response under strong coupling conditions
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Dissociation slowdown by collective optical response under strong coupling conditions

机译：Dissociation slowdown by collective optical response under strong coupling conditions

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摘要

We consider an ensemble of diatomic molecules resonantly coupled to a resonant optical cavity under strong coupling conditions at normal incidence. Photodissociation dynamics is examined via direct numerical integration of the coupled Maxwell-Schrodinger equations with molecular ro-vibrational degrees of freedom explicitly taken into account. It is shown that the dissociation is significantly affected (slowed down) when the system is driven at its polaritonic frequencies. The observed effect is demonstrated to be of transient nature and has no classical analog. An intuitive explanation of the dissociation slowdown at polaritonic frequencies is proposed.

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