Shear enhancement of mechanical and microstructural properties of synthetic graphite and ultra-high molecular weight polyethylene carbon composites

Favreau Hannah J.; Miroshnichenko Kateryna I; Solberg Peder C.Tsukrov Igor I.Van Citters Douglas W.

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Shear enhancement of mechanical and microstructural properties of synthetic graphite and ultra-high molecular weight polyethylene carbon composites

机译：Shear enhancement of mechanical and microstructural properties of synthetic graphite and ultra-high molecular weight polyethylene carbon composites

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Ultra-high molecular weight polyethylene (UHMWPE) has a variety of industrial and clinical applications due to its superb mechanical properties including ductility, tensile strength, and work-to-failure. The versatility of UHMWPE is hindered by the difficulty in processing the polymer into a well consolidated material. This study presents on the effects of shear imparted by equal channel angular pressing (ECAP) on UHMWPE composites containing Nano27 Synthetic Graphite (N27SG). Ductility and work-to-failure improvements up to similar to 60-80% are obtained in sheared N27SG-UHMWPE composites as compared to non-sheared N27SG-UHMWPE controls of the same composition. Microscopy reveals increased fusion at particle boundaries and smaller voids in the sheared materials. Micro-computed tomography results indicate different distribution of N27SG particulates in ECAP samples as compared to CM indicating enhanced grain boundary interactions. Tradeoffs are not avoided as ECAP samples were lower in conductivity as compared to compression molded (CM) billets of the same weight percent. However, ECAP samples were able to be doped with more N27SG allowing for an similar to 170% increase in conductivity over CM samples of the same work-to-failure. This work shows that ECAP is a viable processing method for obtaining stronger, more ductile conductive composite materials.

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来源
《Journal of Applied Polymer Science》 |2022年第20期|共15页
作者
Favreau Hannah J.; Miroshnichenko Kateryna I; Solberg Peder C.Tsukrov Igor I.Van Citters Douglas W.;
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作者单位

Dartmouth Coll;

Univ New Hampshire;

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原文格式 PDF
正文语种英语
中图分类高分子化合物工业（高聚物工业）;
关键词
equal channel angular pressing; nano27 synthetic graphite; ultra-high molecular weight polyethylene; CHANNEL ANGULAR EXTRUSION; GRAPHENE; UHMWPE; WEAR; BIOCOMPATIBILITY; CONSOLIDATION; EXFOLIATION; PERFORMANCE; NANOTUBES;

Shear enhancement of mechanical and microstructural properties of synthetic graphite and ultra-high molecular weight polyethylene carbon composites

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