Binary Organic Solar Cells Breaking 19 via Manipulating the Vertical Component Distribution

Yanan Wei; Zhihao Chen; Guanyu LuNa YuCongqi LiJinhua GaoXiaobin GuXiaotao HaoGuanghao LuZheng TangJianqi ZhangZhixiang WeiXin ZhangHui Huang

首页> 外文期刊>Advanced Materials >Binary Organic Solar Cells Breaking 19 via Manipulating the Vertical Component Distribution

【24h】

Binary Organic Solar Cells Breaking 19 via Manipulating the Vertical Component Distribution

机译：Binary Organic Solar Cells Breaking 19 via Manipulating the Vertical Component Distribution

获取原文

获取原文并翻译 | 示例

掌桥外文数据库（机构版） >>

开具论文收录证明 >>

文献代查 >>

页面导航

摘要
著录项
相关主题

摘要

The variation of the vertical component distribution can significantly influencethe photovoltaic performance of organic solar cells (OSCs), mainly dueto its impact on exciton dissociation and charge-carrier transport and recombination.Herein, binary devices are fabricated via sequential deposition (SD)of D18 and L8-BO materials in a two-step process. Upon independently regulatingthe spin-coating speeds of each layer deposition, the optimal SD deviceshows a record power conversion efficiency (PCE) of 19.05 for binary singlejunctionOSCs, much higher than that of the corresponding blend casting(BC) device (18.14). Impressively, this strategy presents excellent universalityin boosting the photovoltaic performance of SD devices, exemplified byseveral nonfullerene acceptor systems. The mechanism studies reveal thatthe SD device with preferred vertical components distribution possesses highcrystallinity, efficient exciton splitting, low energy loss, and balanced chargetransport, resulting in all-around enhancement of photovoltaic performances.This work provides a valuable approach for high-efficiency OSCs, sheddinglight on understanding the relationship between photovoltaic performanceand vertical component distribution.

著录项

来源
《Advanced Materials》 |2022年第33期|2204718.1-2204718.8|共8页
作者
Yanan Wei; Zhihao Chen; Guanyu LuNa YuCongqi LiJinhua GaoXiaobin GuXiaotao HaoGuanghao LuZheng TangJianqi ZhangZhixiang WeiXin ZhangHui Huang;
展开▼
作者单位

College of Materials Science and Opto-Electronic Technology & Centerof Materials Science and Optoelectronics Engineering & CAS Center forExcellence in Topological Quantum Computation & CAS Key Laboratoryof Vacuum PhysicUniversity of Chinese Academy of Sci;

School of PhysicsState Key Laboratory of Crystal MaterialsShandong UniversityJinan, Shandong 250100, China;

Frontier Institute of Science and TechnologyXi’an Jiaotong UniversityXi’an 710054, ChinaCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620, ChinaKey Laboratory of Nanosystem and Hierarchical FabricationNational Center for Nanoscience and TechnologyBeijing 100190, China;

展开▼
收录信息
原文格式 PDF
正文语种英语
中图分类
关键词
binary organic solar cells; power conversion efficiency; sequential deposition; vertical component distribution;

Binary Organic Solar Cells Breaking 19 via Manipulating the Vertical Component Distribution

摘要

著录项

相关主题

期刊订阅