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Machine learning-assisted design of flow fields for redox flow batteries

机译:Machine learning-assisted design of flow fields for redox flow batteries

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摘要

Flow fields are a crucial component of redox flow batteries (RFBs). Conventional flow fields, designed by trial-and-error approaches and limited human intuition, are difficult to optimize, thus limiting the performance of RFBs. Here, we develop an end-to-end approach to the design of flow fields by combining machine learning and experimental methods. A library of 11 564 flow fields is generated using a custom-made path generation algorithm, in which flow fields are elegantly encoded by two-dimensional binary images. To accelerate the discovery process, we train convolutional neural networks with low test errors for predicting the uniformity factor and pressure drop of flow fields (0.59 and 1.37, respectively). Through a collaborative screening process, eight promising candidates are successfully identified. Experimental validation shows that the battery with the flow fields designed with this approach yields higher electrolyte utilization and exhibits about a 22 increase in limiting current density and up to 11 improvement in energy efficiency compared to the conventional serpentine flow field. Furthermore, statistical analysis suggests that the promising candidates have a saved channel length of 1490 +/- 100 and a torque integral of 20.1 +/- 1.8, revealing the quantitative design rules of flow fields for the first time.

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  • 来源
    《Energy & environmental science: EES》 |2022年第7期|2874-2888|共15页
  • 作者单位

    Hong Kong Univ Sci & Technol, Dept Mech & Aerosp Engn, Kowloon, Clear Water Bay, Hong Kong, Peoples R China;

    Tianjin Univ, Key Lab Efficient Utilizat Low & Medium Grade Ene, Tianjin, Peoples R China|Hong Kong Univ Sci & Technol, Inst Adv Study, Kowloon, Clear Water Bay, Hong Kong, Peoples R China;

    Univ Victoria, Dept Mech Engn, Victoria, BC, Canada|Univ Victoria, Inst Integrated Energy Syst, Victoria, BC, Canada;

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