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Customizable Supercapacitors via 3D Printed Gel Electrolyte

机译:Customizable Supercapacitors via 3D Printed Gel Electrolyte

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摘要

New manufacturing strategies toward customizable energy storage devices(ESDs) are urgently required to allow structural designability for space andweight-sensitive electronics. Besides the macroscopic geometry customization,the ability to fine-tune the ESD internal architectures are key to deviceoptimization, allowing short and uniform electrons/ions diffusion pathwaysand increased contact areas while overcoming the issues of long transportdistance and high interfacial resistance in conventional devices with planarthick electrodes. ESDs with 2D or 3D electrodes filled with liquid or gel-likeelectrolyte have been reported, yet they face significant challenges in designflexibility for 3D ESD architectures. Herein, a novel method of assemblingESDs with the ability to customizing both external and internal architecturesvia digital light processing (DLP) technique and a facile sequential dip-coatingprocess is demonstrated. Using supercapacitors as prototype device, the3D printing of ESDs with areal capacity of 282.7 mF cm~(?2) which is higherthan a reference device with same mass loading employing planar stackedconfiguration (205.5 mF cm~(?2)) is demonstrated. The printed devices withhighly customizable external geometry conveniently allow the ESDs to serveas structural components for various electronics such as watchband andbiomimetic electronics which are difficult to be manufactured with previouslyreported strategies.

著录项

  • 来源
    《Advanced functional materials》 |2023年第20期|2214301.1-2214301.8|共8页
  • 作者单位

    School of Materials Science and EngineeringZhejiang UniversityHangzhou, Zhejiang 310027, P. R. China,Key Laboratory of 3D Micro/Nano Fabrication and Characterizationof Zhejiang ProvinceResearch Center for Industries of the Future and School of Engineering;

    School of Chemistry and Materials ScienceHubei Engineering UniversityHubei 432000, P. R. China,International School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070, P. R. China;

    School of Electronics and InformationHangzhou Dianzi UniversityHangzhou 310018, P. R. ChinaKey Laboratory of 3D Micro/Nano Fabrication and Characterizationof Zhejiang ProvinceResearch Center for Industries of the Future and School of EngineeringWestlake UniversityHangzhou, Zhejiang 310024, P. R. China,Institute of Advanced TechnologyWestlake InAdvanced Materials Additive Manufacturing Research & InnovationCenterSchool of EngineeringZhejiang University City CollegeHangzhou 310015, P. R. China;

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  • 原文格式 PDF
  • 正文语种 英语
  • 中图分类
  • 关键词

    3D printed electrolytes; customizable architectures; structural supercapacitors;

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