Metalloporphyrin-Based Porous Coordination Polymers: Synthesis, Served as Heterogenous Catalysts and Dye Scavengers

Sun Shu; Yu Qiong; Zhang WeiZhao XinLi JunZhang Fengxing

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Metalloporphyrin-Based Porous Coordination Polymers: Synthesis, Served as Heterogenous Catalysts and Dye Scavengers

机译：Metalloporphyrin-Based Porous Coordination Polymers: Synthesis, Served as Heterogenous Catalysts and Dye Scavengers

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Six metalloporphyrin-based porous coordination polymers, Mn-II(TCP)-Mn-II (CP1), Fe-III(TCP)-Fe-III (CP2), Co-II(TCP)-Co-II (CP3), Ni-II(TCP)-Ni-II (CP4), Cu-II(TCP)-Cu-II (CP5) and Zn-II(TCP)-Zn-II (CP6), (TCP = 5,10,15,20-tetra(4-(phenoxy-4-yl)butanoic acid)porphyrin tetravalent anion) were prepared and characterized. CP1, CP2, CP3, CP4 and CP6 are amorphous aggregation supported by SEM, TEM and powder XRD. CP5 is a small particles aggregation with lower crystallinity. These coordination polymers exhibit effective dye scavenging and catalytic activities toward the oxidation of alkylbenzene to ketones, and can be reused by filtration with slight decreasing of catalytic activities.

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来源
《Catalysis Letters》 |2017年第1期|228-239|共12页
作者
Sun Shu; Yu Qiong; Zhang WeiZhao XinLi JunZhang Fengxing;
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作者单位

Northwest Univ, Coll Chem & Mat Sci, Key Lab Synthet & Nat Funct Mol Chem, Minist Educ, Xian 710069, Shaanxi, Peoples R China;

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正文语种英语
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Metalloporphyrin; Alkylbenzene oxidation; Tert-butyl hydroperoxide; Heterogeneous catalytic; Dye scavenger;

Metalloporphyrin-Based Porous Coordination Polymers: Synthesis, Served as Heterogenous Catalysts and Dye Scavengers

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