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首页> 外文期刊>Physical review, B. Condensed matter and materials physics >Impact of orbital degrees of freedom on geometrical frustration in the kagome-like magnet SrVxGa12-xO19
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Impact of orbital degrees of freedom on geometrical frustration in the kagome-like magnet SrVxGa12-xO19

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摘要

We studied kagome-like magnets, SrVxGa12xO19 with V3+ 3d2 in the triply degenerate t2g states, as a geometrically frustrated spin system with orbital degrees of freedom. We observed a suppression of lowtemperature spin entropy and an anomalous contraction of the V triangles on the kagome lattice, which can be regarded as the V trimerization with spin-singlet formation. This result, which is in clear contrast to their Cr3+ 3d3 analogs exhibiting a spin-liquid behavior, indicates a substantial impact of orbitals on geometricallyfrustrated magnets.

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