Growth thermodynamics of nanowires and its application to polytypism of zinc blende Ⅲ-V nanowires

V. G. Dubrovskii; N. V. Sibirev

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Growth thermodynamics of nanowires and its application to polytypism of zinc blende Ⅲ-V nanowires

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Theoretical model for the growth thermodynamics of nanowires in different epitaxial techniques is presented, which enables one to determine morphological and structural configurations of the nanowire ensemble with minimum formation energy. It is demonstrated that nanowire ensembles are metastable and controlled entirely by the growth kinetics. The model is applied to studying the polytypism of zinc blende III-V nanowires. It is shown that structural transition should occur within a certain domain of radii and vapor supersatu-rations. Different polytypes between wurtzite and zinc blende structures with periodicity up to 18 layers are analyzed. It is demonstrated that AH polytype has the lowest formation energy and the largest critical radius of transition amongst all polytypes. Numerical estimates predict the critical radius of structural phase transition of 17-25 nm for GaAs nanowires growing on the GaAs(111)B substrate.

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《Physical review, B. Condensed matter and materials physics》 |2008年第3期|035414.1-035414.8|共9页
作者
V. G. Dubrovskii; N. V. Sibirev;
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St. -Petersburg Physical Technological Centre of the Russian Academy of Sciences for Research and Education, Khlopina 8/3, 195220 St.-Petersburg, Russia;

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正文语种英语
中图分类固体物理学;
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theory and models of crystal growth; physics of crystal growth; crystal morphology and orientation; whiskers and dendrites (growth; structure; and nonelectronic properties);

Growth thermodynamics of nanowires and its application to polytypism of zinc blende Ⅲ-V nanowires

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