Energy spectra of Hminus;ions from a HDD source operating in mixtures of helium, hydrogen, and cesium reveal that negative ions are generated by a volume process and by a surface process. A marked difference was observed in the pressure dependence of the lowhyphen; and highhyphen;energy groups, corresponding to the volume and the surface processes, respectively. The active surfaces could be identified. Some evidence that, besides collisional attachment processes, ionhyphen;molecular reactions have an influence on the yield of Hminus;ions in volume reactions could be found.
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