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The influence of phase fluctuations and phase modulation on two-photon fluorescence

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In the present paper the two-photon fluorescence (TPF) quenching produced by ruby lasers in dye is calculated on the basis of an electronic energy level system adapted for the special conditions of Rhodamine 6G. The model used here takes into consideration the action of competing one-photon processes. It will be shown that the reversed profile of TPF quenching in the overlap region is produced by the superposition of pulses with a time-dependent fluctuating phase as well as with a determinate quadratically time-dependent phase.

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