Selective isopentane formation from CH3OH on a new one-atomic layer ZrO2/ZSM-5 hybrid catalyst

KiyotakaAsakura; MutsutoAoki; YasuhiroIwasawa

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Selective isopentane formation from CH3OH on a new one-atomic layer ZrO2/ZSM-5 hybrid catalyst

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A new one-atomic layer ZrO2/ZSM-5 hybrid catalyst was prepared by using the repeated reactions between Zr(OC2H5)4and of the OH groups of the external surfaces of ZSM-5, followed by calcination. The one-atomic layer ZrO2attached on the ZSM-5 surface was characterized by means of X-ray diffraction, X-ray fluorescence and EXAFS. The ZrO2overlayer is suggested to epitaxially grow on the ZSM-5(001) plane in a 111 direction of tetragonal ZrO2. The one-atomic layer ZrO2/ZSM-5 is a unique catalyst which produces selectively isopentane from CH3OH.

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《catalysis letters》 |1988年第11期|395-403|共页
作者
KiyotakaAsakura; MutsutoAoki; YasuhiroIwasawa;
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the University of Tokyo;

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Selective isopentane formation from CH3OH on a new one-atomic layer ZrO2/ZSM-5 hybrid catalyst

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