Carbazolo2,1-acarbazole Diimide: A Building Block for Organic Electronic Materials

Zhao Zheng; Wang Zhongli; Zhang XuGao SiminYang XiaodiDuan ZhimingGao Xike

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Carbazolo2,1-acarbazole Diimide: A Building Block for Organic Electronic Materials

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A new class of carbazolo2,1-acarbazole diimide compounds (CBZCBZ-DI, 3) are designed and synthesized. The synthesis, X-ray crystal structure, absorption spectra, and electrochemical properties of 3 as well as the charge transport properties are investigated. Theoretical calculation is also carried out based on the X-ray crystal structure of 3a to understand the relationship between the structure and the charge transport properties. Single-crystal X-ray analysis revealed that the molecules of 3a adopt a slipped face-to-face pi-stacking mode with a large intermolecular pi-overlap and an interplanar distance of 3.4 angstrom. Crystalline transistors of 3a display high hole mobility of 0.5 cm(2)V(-1) s(-1), which is among the highest reported mobility values for carbazole-based N-heteroacenes. Two useful brominated derivatives (4, 5) are also prepared for synthesizing more new pi-functional materials.

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来源
《ChemPlusChem》 |2015年第1期|57-61|共5页
作者
Zhao Zheng; Wang Zhongli; Zhang XuGao SiminYang XiaodiDuan ZhimingGao Xike;
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作者单位

Chinese Acad Sci, Shanghai Inst Organ Chem, Key Lab Synthet & Self Assembly Chem Organ Funct;

Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China;

Shanghai Univ, Dept Chem, Shanghai 200444, Peoples R China;

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原文格式 PDF
正文语种英语
中图分类化学;
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carbazoles; crystalline transistors; density functional calculations; diimides;

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Carbazolo2,1-acarbazole Diimide: A Building Block for Organic Electronic Materials

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