Photoinduced charge transfer involving a MoMo quadruply bonded complex to a perylene diimide

Alberding B.G.; Brown-Xu S.E.; Chisholm M.H.Epstein A.J.Gustafson T.L.Lewis S.A.Min Y.

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Photoinduced charge transfer involving a MoMo quadruply bonded complex to a perylene diimide

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Evidence, based on femtosecond transient absorption and time resolved infrared spectroscopy, is presented for photoinduced charge transfer from the Mo_2δ orbital of the quadruply bonded molecule trans-Mo _2(TiPB)_2(BTh)_2, where T iPB = 2,4,6-triisopropyl benzoate and BTh = 2,2′- bithienylcarboxylate, to di-n-octyl perylene diimide and di-n-hexylheptyl perylene diimide in thin films and solutions of the mixtures. The films show a long-lived charge separated state while slow back electron transfer, τ_(BET) ～ 500 ps, occurs in solution.

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《Dalton transactions: An international journal of inorganic chemistry》 |2013年第15期|5275-5280|共6页
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Alberding B.G.; Brown-Xu S.E.; Chisholm M.H.Epstein A.J.Gustafson T.L.Lewis S.A.Min Y.;
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Ohio State University, 100 West 18th Avenue, Columbus, OH 43210, United States;

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中图分类化学;
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Photoinduced charge transfer involving a MoMo quadruply bonded complex to a perylene diimide

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