Phenol ring nitration induced by the unprecedented reduction of the Cu(ii) centre by nitrogen dioxide

Kumar V.; Kalita A.; Mondal B.

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Phenol ring nitration induced by the unprecedented reduction of the Cu(ii) centre by nitrogen dioxide

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Nitrogen dioxide (NO_2) induces tyrosine nitration through a radical mechanism in biological systems. Two copper(ii) complexes, 1 and 2, with ligands L_1 and L_2 L_1 = 2,4-di-tert-butyl-6- (((2-(dimethylamino)ethyl)(isopropyl)amino)methyl)phenol; L_2 = 6,6′-(((2-(dimethylamino)ethyl)azanediyl)bis(methylene))bis(2, 4-di-tert-butylphenol), respectively, have been made to react with NO 2. In both cases, the reduction of the copper(ii) center was observed in the presence of NO_2 which induces phenol ring nitration through nitronium ion (NO_2~+) formation.

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来源
《Dalton transactions: An international journal of inorganic chemistry》 |2013年第46期|16264-16267|共4页
作者
Kumar V.; Kalita A.; Mondal B.;
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作者单位

Department of Chemistry, Indian Institute of Technology, Guwahati Assam 781039, India;

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原文格式 PDF
正文语种英语
中图分类化学;无机化学;
关键词
Copper complexes; Nitrogen dioxides; Nitronium;

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Phenol ring nitration induced by the unprecedented reduction of the Cu(ii) centre by nitrogen dioxide

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