Two birds with one stone: Anion templated ball-shaped Ag_(56) and disc-like Ag_(20) clusters

Sun D.; Wang H.; Lu H.-F.Feng S.-Y.Zhang Z.-W.Sun G.-X.Sun D.-F.

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Two birds with one stone: Anion templated ball-shaped Ag_(56) and disc-like Ag_(20) clusters

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One-pot reaction of AgSBu~t and AgOAc in the methanol-ethanol-DMF solvent system under room temperature gave a ball-shaped Ag_(56) cluster and a disc-like Ag_(20) cluster. The formations of clusters 1 and 2 are templated by an in situ generated S~(2-) ion from the cleavage of the S-C bond of SBu~t and CO_3 ~(2-) ion from the fixation of atmospheric carbon dioxide, respectively. Interestingly, cluster 1 only emits bright-red light in the solid state at 77 K and is not emissive at room temperature.

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《Dalton transactions: An international journal of inorganic chemistry》 |2013年第18期|6281-6284|共4页
作者
Sun D.; Wang H.; Lu H.-F.Feng S.-Y.Zhang Z.-W.Sun G.-X.Sun D.-F.;
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作者单位

Key Laboratory of Special Functional Aggregated Materials, Ministry of Education, Shandong University, Jinan 250100, China;

School of Chemistry and Chemical Engineering, University of Jinan, 106 Jiwei Road, 250022 Jinan, China;

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正文语种英语
中图分类化学;
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AgOAc; ball-shaped; atmospheric;

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Two birds with one stone: Anion templated ball-shaped Ag_(56) and disc-like Ag_(20) clusters

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