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Modeling of CO2 absorption in membrane contactors

机译:膜接触器中二氧化碳吸收的建模

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A comprehensive two-dimensional mathematical model was developed for the transport of carbon dioxide through hollow fiber membrane(HFM)contactors.The model was based on"non-wetted mode"in which the gas mixture filled the membrane pores for countercurrent gas-liquid contact.Laminar parabolic velocity profile was used for the gas flow in the tube side;whereas,the liquid flow in the shell side was characterized by Happel's free surface model.Axial and radial diffusion inside the fiber,through the membrane,and within the shell side of the contactor were considered in the model.Moreover,the model was validated with the experimental results obtained for carbon dioxide removal from CO2/CH4 gas mixture using polypropylene membrane contactor with distilled water as the liquid solvent.The modeling predictions were in good agreement with the experimental results for different values of gas and liquid flow rate,gas to liquid ratio,and temperature.
机译:建立了用于中空纤维膜(HFM)接触器的二氧化碳传输的综合二维数学模型。该模型基于“非润湿模式”,其中气体混合物充满膜孔以进行逆流气液接触管的气体流动采用层流抛物线速度分布;而壳的液体流动则采用Happel的自由表面模型来表征。纤维内部,通过膜以及壳内部的轴向和径向扩散在模型中考虑了接触器的特性。此外,该模型还得到了以蒸馏水为液体溶剂的聚丙烯膜接触器从CO2 / CH4气体混合物中脱除二氧化碳的实验结果进行验证。在不同的气液流量,气液比和温度值下的实验结果。

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