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Coherent Raman Mixing and Coherent Anti-Stokes Raman Scattering from Individual Micrometersize Droplets

机译:单个微米级液滴的相干拉曼混合和相干反斯托克斯拉曼散射

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摘要

The coherent Raman mixing spectra from individual micrometer-sized droplets of ethanol and of water consist of regularly spaced peaks that correspond to the morphology dependent resonances of a spherical droplet. In contrast, the coherent anti Stokes Raman scattering spectra from droplets exhibit no morphology dependent peaks. Both results are explained by the spatial overlap of the enhanced internal field distributions and by the phase matching conditions associated with the droplet. Keywords: Reprints; Coherent anti-Strokes Raman scattering; Stimulated Raman scattering; Morphology dependent resonances; Phase matching angle; Vibrating orifice generator; Liquid droplets; Coherent Raman Mixing; Four wave mixing process; Liquid air interface.

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