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Non-Equilibrium Kinetics: Explicit Time-Dependence Of Perturbed Distribution Functions and Auto-Correlation Expressions

机译：非平衡动力学：扰动分布函数和自相关表达式的显式时间依赖性

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摘要

The explicit time dependence of perturbed distribution functions is considered for a chemically reacting dilute gas mixture. The solutions obtained for the distribution functions approach in time the normal solutions of a Chapman-Enskog perturbation treatment within a few mean free times, and provide an auto-correlation expression for the first non-equilibrium correction to the rate coefficient for a bimolecular gas phase reaction. To illustrate the results, explicit solutions are obtained for two model systems. (Author)

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Kapral, R.; Hudson, S.; Ross, J.;
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年度 1970
页码 p.1-29
总页数 29
原文格式 PDF
正文语种 eng
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关键词
Reaction kinetics ; Gases ; Chemical reactions ; Statistical mechanics ; Chemical equilibrium;

机译：反应动力学;气体;化学反应;统计力学;化学平衡;

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Non-Equilibrium Kinetics: Explicit Time-Dependence Of Perturbed Distribution Functions and Auto-Correlation Expressions

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