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Catalytic and Surface Science Studies of Clean and Modified Rhodium, Molybdenum and Palladium Crystal Surfaces: Hydrogenation of Carbon Monoxide and the Cyclotrimerization of Acetylene to Form Benzene

机译：清洁和改性铑，钼和钯晶体表面的催化和表面科学研究：一氧化碳的加氢和乙炔的环三聚反应形成苯

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The effect of additives on catalysts for the hydrogenation of carbon monoxide and the cyclotromerization of acetylene has been investigated using both low pressure surface science techniques and high pressure reaction studies. Additives were found to have relatively complicated catalytic behavior, which could be explained with the aid of surface analytical tools such as AES, XPS, TPD, and LEED. Potassium was found to have the greatest effect on both the hydrogenation of CO and the cyclotrimerization of acetylene over all metal catalysts. For CO hydrogenation over Rh, a large equilibrium deuterium isotope effect was observed. (ERA citation 12:000972)

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作者
Logan, M. A.;
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年度 1985
页码 1-258
总页数 258
原文格式 PDF
正文语种 eng
中图分类工业技术;
关键词
Acetylene; Carbon Monoxide; Deuterium; Molybdenum; Palladium; Rhodium; Additives; Catalysts; Catalytic Effects; Hydrogenation; Isotope Effects; Monocrystals; Polymerization; Potassium; Surfaces;

机译：乙炔;一氧化碳;氘;钼;钯;铑;添加剂;催化剂;催化作用;加氢;同位素效应;单晶;聚合;钾;表面;

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专利

1. Vibrational Study of the Interaction of Acetylene and Benzene on Clean and Carbide-Modified W(211) Surfaces [J] . J. Eng Jr., J. G. Chen, I. M. Abdelrehim, The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 1998,第48期

机译：乙炔和苯在清洁和碳化物修饰的W（211）表面上相互作用的振动研究
2. Vibrational Study of the Interaction of Acetylene and Benzene on Clean and Carbide-Modified W(211) Surfaces [J] . J. Eng, Jr., J. G. Chen The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 1998,第45a48期

机译：乙炔和苯在清洁和碳化物修饰的W（211）表面上相互作用的振动研究
3. Surface reactions on inverse model catalysts: CO adsorption and CO hydrogenation on vanadia-and ceria-modified surfaces of rhodium and palladium [J] . Konrad Hayek, Bernd Jenewein, Bernhard Klotzer Topics in Catalysis . 2001,第1a4期

机译：逆模型催化剂的表面反应：钒和二氧化铈修饰的铑和钯表面上的CO吸附和CO加氢
4. Catalytic Formation of Carbon-Carbon Bonds in Ultrahigh Vacuum: Cyclotrimerization of Alkynes on Reduced TiO_2 Surfaces [C] . K. G. Pierce, V.S. Lusvardi, M.A. Barteau International congress on catalysis;ICC . 1996

机译：超高真空下碳-碳键的催化形成：还原的TiO_2表面上炔烃的环三聚
5. In situ mechanistic studies of the oxidation of carbon monoxide, ethylene, and acetylene over platinum surfaces. [D] . Burnett, Daniel James. 2001

机译：铂表面上一氧化碳，乙烯和乙炔氧化的原位机理研究。
6. X-ray photoemission analysis of clean and carbon monoxide-chemisorbed platinum(111) stepped surfaces using a curved crystal [O] . Andrew L. Walter, Frederik Schiller, Martina Corso, -1

机译：使用曲面晶体对清洁的和一氧化碳化学吸附的Platinum（111）台阶表面进行X射线光发射分析
7. The effect of additives on the reactivity of palladium surfaces for the chemisorption and hydrogenation of carbon monoxide: A surface science and catalytic study. LaMO/sub 3/(M = Cr, Mn, Fe, Co, Rh) [O] . T.G. Rucker 1987

机译：添加剂对钯表面对二氧化碳化学和氢化的影响的影响：表面科学与催化研究。 Lamo / Sub 3 /（M = Cr，Mn，Fe，Co，Rh）
8. Effect of Additives on the Reactivity of Palladium Surfaces for the Chemisorption and Hydrogenation of Carbon Monoxide: A Surface Science and Catalytic Study [R] . Rucker, T. G. 1987

机译：添加剂对钯表面对一氧化碳化学吸附和加氢反应性的影响：表面科学和催化研究

Catalytic and Surface Science Studies of Clean and Modified Rhodium, Molybdenum and Palladium Crystal Surfaces: Hydrogenation of Carbon Monoxide and the Cyclotrimerization of Acetylene to Form Benzene

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