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Application of the ESCIMO Theory to the Oxidation of Methane in a Stirred Reactor

机译:EsCImO理论在搅拌反应器中甲烷氧化反应中的应用

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摘要

An investigation into the reaction between methane and air under turbulent conditions in a stirred reactor is proposed. Problems arising in the modeling of turbulent flows involving exothermic chemical reaction are outlined and different approaches to a solution are reviewed. The ESCIMO theory is described. A computer code which applies the ESCIMO theory to the biographic features of the multistep hydrogen-oxygen reaction is outlined and the changes necessary for program adaption to methane-air reaction are discussed. Experimental studies on the chemical kinetics and flame propagation of the methane-air system are reviewed. Results from computer simulations on near stoichiometric methane-air mixtures reflect the existence of laminar flame speed control, stretching control, and chemical kinetics control burning regimes. Grid independence tests and step size control tests carried out on stretching regime indicate a cross stream grid of 40 nodes is acceptable.

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