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Production of synthesis gas from natural gas with copper—iron—manganese oxide oxygen carriers/catalysts via partial oxidation and dry reforming processes
Production of synthesis gas from natural gas with copper—iron—manganese oxide oxygen carriers/catalysts via partial oxidation and dry reforming processes
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机译：通过部分氧化和干燥重整过程从铜 - 铁 - 锰氧化物氧载体/催化剂的天然气生产合成气
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摘要
Materials, methods of making, and methods of providing a trimetallic oxygen carrier for converting methane containing fuel to synthesis gas. The trimetallic oxygen carrier comprises CuxFeyMnzOt, where CuxFeyMnzOt is a chemical composition with 0xFeyMnzOt may be one of CuMnFeO4, CuFe0.5Mn1.5O4, CuFeMn2O4, CuFe2MnO4, or Cu impregnated on FerMnsOu, Fe impregnated on CurMnsOu, Mn impregnated on CurFesOu where r>0, s>0 and u>0 and combinations thereof. Reaction of trimetallic CuxFeyMnzOt with methane generates a product stream comprising at least 50 vol. % CO and H2.
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机译：材料，制备方法以及提供用于将含甲烷的三种子氧载体转化为合成气的方法。三相氧载体包含Cu x fe y mn z O t ，其中Cu x Fe Y Mn z O t 是一种化学组合物，0 x fe y mn z O t 可以是cumnfeo 4 ，CUFE 0.5 Mn 1.5 O 4 ，CUFEMER 2 O 4 ， CUFE 2 mno 4 ，或浸渍在fermnsou，Fe浸渍在Curmnsou上的Fe，Mn浸渍在Curfesou上，其中R> 0，S> 0和U> 0及其组合。三种金属Cu X / sub> Fe Y Mn z O t 用甲烷产生至少50 vol的产物流。 ％co和h 2 。
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