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首页> 外文会议>Advances in structures, properties and applications of biological and bioinspired materials >Effect of Microtubules Hierarchy on Photoinduced Hydrogen Generation and Application to Artificial Photosynthesis
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Effect of Microtubules Hierarchy on Photoinduced Hydrogen Generation and Application to Artificial Photosynthesis

机译：微管层次对光诱导氢产生的影响及其在人工光合作用中的应用

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摘要

Several strategies have been explored from viewpoint of biomimetics to accomplish artificial photosynthesis by using macromolecules as a medium such as liposomes, supramolecules, and hydrogels. Differing from disordered solution systems in which multiple components such as photosensitizer and catalytic nanoparticle are diffusively mixed, the photochemical reactions occur efficiently in medium due to maintenance of the dipersibility of the components and specific molecular arrangement. Here we attempt to clarify the effect of medium hierarchy for photoinduced electronic transmission among multiple components. By conjugating each component on tubulin and integrating them via self-assembly to microtubules, ideal component arrangements with optimum distance for the electronic transmission will be possible.
机译：从仿生学的观点出发，已经探索了几种通过使用大分子作为脂质体，超分子和水凝胶等介质来完成人工光合作用的策略。与其中多种组分（例如光敏剂和催化纳米颗粒）扩散混合的无序溶液系统不同，由于保持了组分的可分散性和特定的分子排列，光化学反应在介质中有效地发生。在这里，我们试图阐明介质层次对于多个组件之间的光感应电子传输的影响。通过将微管蛋白上的每个成分结合在一起，并通过自组装将它们整合到微管中，可以实现具有最佳距离的理想组件排列，以实现电子传输。

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  • 会议地点 Boston MA(US)
  • 作者

    Kosuke Okeyoshi; Kawamura Ryuzo; Ryo Yoshida; Yoshihito Osada;

  • 作者单位

    RIKEN Advanced Science Institute, 2-1 Hirosawa Wako-shi, Saitama 351-0198, Japan,Department of Materials Engineering, Graduate School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo, 113-8656, Japan;

    RIKEN Advanced Science Institute, 2-1 Hirosawa Wako-shi, Saitama 351-0198, Japan;

    Department of Materials Engineering, Graduate School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo, 113-8656, Japan;

    RIKEN Advanced Science Institute, 2-1 Hirosawa Wako-shi, Saitama 351-0198, Japan;

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