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Morphological Characterization of Atmospheric Aggregates

机译:大气聚集体的形态表征

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Many ultrafine atmospheric aerosol particles have aggregate structures. Thernmorphological properties of atmospheric aggregates are important for understanding theirrnsources, transport, and health risk. Atmospheric aggregates can be characterized in partrnusing fractal concepts. In this study, particles were collected on the transmission electronrnmicroscope grids placed on the lower stages (7 and 8) of a low-pressure Hering impactor.rnMost of the particles deposited on these stages were fractal-like. The particles arernanalyzed under the transmission electron microscope. Computer programs were used tornfind fractal dimension from the primary particle sizes and location. In the analysis ofrnparticles composed of 10 to 180 primary particles, the number of primary particles andrnfractal dimension (D_f) have an approximately linear relationship for Df values rangingrnfrom near unity to above 2. The atmospheric particles were also compared to soot andrnsimulated aggregates, in terms of their fractal dimension and primary particle sizerndistribution. Although the basic structures are similar, the primary particles making uprnthe aggregates vary between the soot and atmospheric particles.
机译:许多超细大气气溶胶颗粒具有聚集结构。大气团聚体的形态学特性对于了解其来源,运输和健康风险非常重要。大气聚集体可以通过分形概念来表征。在这项研究中,颗粒被收集在放置在低压Hering撞击器下段(7和8)的透射电子显微镜格栅上。大多数沉积在这些阶段的颗粒是分形的。在透射电子显微镜下分析颗粒。使用计算机程序从主要粒度和位置中寻找分形维数。在分析由10到180个初级粒子组成的粒子时,初级粒子的数量和分数维(D_f)对于Df值(从近似1到大于2)具有近似线性关系。大气粒子也与烟灰和模拟集料进行了比较的分形维数和初级粒径分布尽管基本结构相似,但构成聚集体的主要颗粒却在烟尘和大气颗粒之间变化。

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