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Colossal Magnetoresistance and Phase Separation in Manganite Thin Films

机译:锰铁薄膜中的巨大磁阻和相分离

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In the present work, polycrystalline Sm_05_5Sr_04_5MnO3 thin films were prepared on LSAT (001) single crystal substrates by ultrasonic nebulized spray pyrolysis technique. The X-ray diffraction θ-2θ scan reveals that these films (i) have very good crystallinity, (ii) are oriented along out-of-plane c-direction, and (iii) are under small tensile strain. The impact of oxygen vacancy results into (i) higher value of paramagnetic insulator (PMI) to ferromagnetic metal (FMM) transition temperature, i.e., T_C/T_(IM), (ii) sharper PMI-FMM transition, (iii) higher value of magnetization and magnetic saturation moment, and (iv) higher value of magnetoresistance (~99%). We suggest here that oxygen vacancy favors FMM phase while oxygen vacancy annihilation leads to antiferromagnetic-charge ordered insulator (AFM-COI) phase. The observed results have been explained in context of phase separation (PS) caused by different fractions of the competing FMM and AFM-COI phases.
机译:在本作工作中,通过超声雾化喷雾热解技术在LSAT(001)单晶基板上制备多晶SM_05_5SR_04_5MNO3薄膜。 X射线衍射θ-2θ扫描显示,这些薄膜(I)具有非常好的结晶度,(ii)沿着面外C方向取向,(III)在小拉伸菌株下。氧空位结果的影响(i)升高的顺磁绝缘体(PMI)对铁磁性金属(FMM)转变温度,即T_C / T_(IM),(II)锐白PMI-FMM转换,(III)更高的值磁化和磁血液饱和矩,(iv)磁阻值较高(〜99%)。我们在此建议氧气空缺率源于FMM阶段,而氧空位湮没导致反铁磁性充电有序绝缘体(AFM-COI)相。已经在竞争的FMM和AFM-COI相位不同的分离(PS)的上下文中解释了所观察结果。

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